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海底地下水排放(SGD)是近海海域的一个重要的营养盐来源。本研究借助多种天然镭同位素对春季苏北浅滩海域的SGD及其携带入海的营养盐通量进行量化评估。研究发现:苏北浅滩海域的~(224)Ra、~(223)Ra和~(226)Ra等镭同位素的浓度水平较高,呈现近岸高、远岸低的分布趋势;根据~(224)Ra/~(226)Ra的"表观年龄模型"估算的水龄的分布情况推断,春季该海域表层水体主体流向为东北向,流速约为0.1m/s,这与前人物理海洋数值模拟结果一致;最终利用226Ra质量平衡模型发现海域的SGD通量为(46±29)cm/d,由其携带入海的溶解态无机氮、磷、硅营养盐(DIN、 DIP、 DSi)等的通量分别为(2.6±3.1)×1~09、(3.0±2.5)×10~6和(5.5±4.2)×10~8mol/d。 相似文献
2.
基于223Ra和224Ra的桑沟湾海底地下水排放通量 总被引：1，自引：0，他引：1
海底地下水排放（SGD）是陆地向海洋输送水量和营养物质的重要通道之一,对沿海物质通量及其生物地球化学循环有重要的影响,对生态环境起着不可忽视的作用。本文运用天然放射性同位素223Ra和224Ra示踪估算了我国北方典型养殖基地桑沟湾的海底地下水排放通量。结果表明,海底地下水样尤其是间隙水中Ra活度[224Ra=（968±31）dpm/（100 L）,223Ra=（31.4±4.9）dpm/（100 L）,n=9]远高于表层海水[224Ra=（38.7±2.0）dpm/（100 L）,223Ra=（1.70±0.50）dpm/（100 L）, n=21]。假设稳态条件下,考虑Ra的各源、汇项,利用Ra平衡模型,估算出桑沟湾SGD排放通量为（0.23~1.03）×107 m3/d。潮周期内的观测结果显示,涨潮时,水力梯度较小,SGD排放变弱,落潮时,水力梯度较大,导致了相对较多的SGD排放。在一个潮周期间,基于223Ra和224Ra得到的SGD排放通量平均为0.39×107 m3/d。潮汐动力下的SGD排放平均占总SGD排放的61%,因此桑沟湾沿岸的地下水排放主要受潮汐动力的影响,并对海水组成及海陆间物质交换有显著贡献。 相似文献
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P.P. Povinec J. de Oliveira E.S. Braga J.-F. Comanducci J. Gastaud M. Groening I. Levy-Palomo U. Morgenstern Z. Top 《Estuarine, Coastal and Shelf Science》2008
Stable isotopes, tritium, radium isotopes, radon, trace elements and nutrients data were collected during two sampling campaigns in the Ubatuba coastal area (south-eastern Brazil) with the aim of investigating submarine groundwater discharge (SGD) in the region. The isotopic composition (δD, δ18O, 3H) of submarine waters was characterised by significant variability and heavy isotope enrichment. The stable isotopes and tritium data showed good separation of groundwater and seawater groups. The contribution of groundwater in submarine waters varied from a few % to 17%. Spatial distribution of 222Rn activity concentration in surface seawater revealed changes between 50 and 200 Bq m−3 which were in opposite relationship with observed salinities. Time series measurements of 222Rn activity concentration in Flamengo Bay (from 1 to 5 kBq m−3), obtained by in situ underwater gamma-spectrometry showed a negative correlation between the 222Rn activity concentration and tide/salinity. This may be caused by sea level changes as tide effects induce variations of hydraulic gradients, which increase 222Rn concentration during lower sea level, and opposite, during high tides where the 222Rn activity concentration is smaller. The estimated SGD fluxes varied during 22–26 November between 8 and 40 cm d−1, with an average value of 21 cm d−1 (the unit is cm3/cm2 per day). The radium isotopes and nutrient data showed scattered distributions with offshore distance and salinity, which implies that in a complex coast with many small bays and islands, the area has been influenced by local currents and groundwater–seawater mixing. SGD in the Ubatuba area is fed by coastal contaminated groundwater and re-circulated seawater (with small admixtures of groundwater), which claims for potential environmental concern with implications on the management of freshwater resources in the region. 相似文献
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福建省漳州市隆教湾海水中镭同位素的研究,目的是评价海底地下水排泄量。在2007年6月的航次中,垂直于岸线的9km剖面上布置15个站位,每个站位用潜水泵采集表层海水样60L于塑料桶中。水样运回实验室后,立即用装有锰纤维的PVC管以虹吸的方式富集水样中的镭同位素,水通过PVC管的流速小于300ml/min。224Ra活度用连续射气法测定,测完224Ra后密封7d以上,然后用直接射气法测定226Ra活度。224Ra和226Ra活度都呈现自岸向海逐渐降低的规律,表明扩散控制镭同位素的分布,由224Ra获得68.83km2d-1的扩散系数,同时226Ra形成-0.963dpm100l-1km-1的活度梯度。用扩散系数和活度梯度建立的226Ra的离岸通量为6.62×1011dpmkm-2d-1,这个通量一定是得到SGD输入的镭支持,从而获得隆教湾的海底地下水排泄量是3.03×109m3km-2d-1。该排泄量包括陆源地下淡水排泄量和再循环海水排泄量,绝大部分可能是再循环海水,有待进一步研究。 相似文献
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本文介绍带电收集片测定土等粉末样品的 Ra 含量来找 U 矿的方法,称为 Ra 法。此法灵敏度高,操作简便,成本低,可以使用~(210)Po 法曲仪器和铜片,便于推广使用。文中介绍了测 Ra 流程,测定误差和灵敏度.Ra 法在详查和区调阶段的用途。总结了深部盲矿、地表矿化和非矿异常地段上地表的 Ra、Po 和γ异常的特征,指明 Ra 法和 Po 法结合可用于评价异常,提高找深部铀矿的能力。 相似文献
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本文采用电离法(平板电离室装置)对英产镭源和苏联产镭源进行了研究,找出了两种不同当量壳镭源之间的相关关系,解决了按照国际镭源标准对苏联产镭源含量的检定方法。 相似文献
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The Subei Shoal is the largest sandy ridge in the southern Yellow Sea and is important source for nutrient loading to the sea. Here, the nutrient fluxes in the Subei Shoal associated with eddy diffusion and submarine groundwater discharge（SGD） were assessed to understand their impacts on the nutrient budget in the Yellow Sea. Based on the analysis of 223 Ra and 224 Ra in the field observation, the offshore eddy diffusivity mixing coefficient and SGD were estimated to be 2.3×108 cm 相似文献
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Guangquan Chen Bochao Xu Shibin Zhao Disong Yang William C.Burnett Shaobo Diao Maosheng Gao Xingyong Xu Lisha Wang 《海洋学报(英文版)》2022,41(1):11-20
Submarine groundwater discharge(SGD) has received increasing attention by studies on coastal areas; however,its effects on biogeochemical zonation have not been investigated to date. The Huanghe River Estuary(HRE) is a world class river estuary with high turbidity, and heavy human regulation. This study investigated how SGD is related to the benthic biogeochemistry of the HRE. Based on the distribution of several parameters(e.g., salinity,temperature, dissolved oxygen(DO) levels, p H, radium iso... 相似文献
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错流超滤技术在海水胶体态铀、钍、镭同位素和有机碳研究中的应用 总被引：17，自引：3，他引：14
建立了由预过滤装置、蠕动泵、中空纤维超滤膜(AmiconH10P10-20,标称截留分子量10KDa)和连接管组成的错流超滤系统,利用荧光标记的40KDa葡聚糖和已知放射性活度的234Th示踪剂评估了超滤膜的截留和吸附性质,探讨了234Th在超滤过程中的渗透行为,考查了该系统用于实际海水样品时铀、钍、镭同位素和有机碳的质量平衡状况.结果表明,10Kda中空纤维超滤膜对40Kda葡聚糖具有良好的截留效率(85%),而吸附损失率为18%.铀、钍、镭同位素和有机碳在超滤过程中均达到极佳的质量平衡,回收率R=95%～98%,优于大多数文献报道的值.234Th在超滤过程中的渗透行为可以很好地用渗透模型加以描述.研究组分胶体态含量占“溶解”态含量的份额大小顺序如下:钍同位素、有机碳、镭同位素约等于铀同位素,这与钍为强颗粒活性元素、铀和镭为水溶性元素的地球化学性质相吻合. 相似文献