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1.
A. A. Krylov O. M. Khlystov T. I. Zemskaya H. Minami A. Hachikubo H. Shoji M. Kida T. P. Pogodaeva L. Naudts J. Poort 《Geochemistry International》2008,46(10):985-995
This paper presents data on authigenic siderite first found in surface sediments from mud volcanoes in the Central (K-2) and Southern (Malen’kii) basins of Lake Baikal. Ca is the predominant cation, which substitutes Fe in the crystalline lattice of siderite. The enrichment of the carbonates in the 13C isotope (from +3.3 to +6.8‰ for the Malen’kii volcano and from +17.7 to +21.9‰ for K-2) results from the crystallization of the carbonates during methane generation via the bacterial destruction of organic matter (acetate). The overall depletion of the carbonates in 18O is mainly inherited from the isotopic composition of Baikal water. 相似文献
2.
Mercury emissions from the incineration of automobile shredder residues (ASRs) were investigated. Continuous monitoring of elemental and reactive gaseous Hg in flue gas was performed in lab-scale and plant-scale ASR incineration. Results of continuous monitoring agreed with those obtained using the JIS K0222 method and Ontario-Hydro method. Before cleaning by air pollutant control devices (APCDs), reactive Hg was the dominant form of that element in both lab-scale and plant-scale results. Emission factors of reactive Hg before APCDs estimated from monitoring results showed large differences between plant-scale and lab-scale emissions. The emission factor in the plant scale was more than 10 times larger than that in the lab-scale, which is explainable by the different Hg contents of ASR. Based on plant-scale monitoring at the stack, emission factors after APCDs were estimated as 0.79 mg-Hg/Mg-ASR for elemental Hg and 6.8 mg-Hg/Mg-ASR for reactive Hg. Using these emission factors, total Hg emissions from ASR incineration were estimated as 2.2 kg/a. An ASR incineration plant investigated in this study used highly effective APCDs. Consequently, these emission factors might result in underestimation of national Hg emissions from ASR incineration. Emission factors estimated from lab-scale monitoring at a fabric filter outlet side might be more appropriate. However, even if emission factors calculated from plant-scale or the lab-scale monitoring are used, estimated emissions are still less than 1.0% of total Hg emissions in Japan. Therefore, Hg emissions from ASR incineration can be evaluated as insignificant. Unless Hg contents of ASR increase extremely, ASR incineration would be a minor source of Hg atmospheric emission in Japan, even if all ASRs were incinerated. 相似文献
3.
A simple indirect method for the determination of organic carbon in marine particulate matter is proposed. The recommended procedure is as follows: The dried sample is ashed at 450°C for about 24 hr. The ashed sample is put into a Teflon vessel followed by a mixed solution of nitric acid, perchloric acid and hydrofluoric acid. The vessel is sealed and allowed to stand at 150°C for 5 hr. The concentrations of Si and Al in the digested solution are determined. The organic carbon content (Cal-C, %) is calculated by the following equation: Cal-C=0.52 ([CF]–0.10 [Opal]–0.03 [A-Si]), where [CF] is the combustible fraction (%), [Opal] is the biogenic-SiO2(%), and [A-Si] is the content of aluminosilicate mineral (%). 相似文献
4.
Sediment trap experiments were carried out 39 times during the years from 1977 to 1981 in Funka Bay, Hokkaido, Japan. The observed total particulate flux varies seasonally, that is, the particulate fluxes in winter and spring are larger than those in summer. The fluxes in all seasons increased with depth. Major components of settling particles are aluminosilicate in winter, biogenic silicate in spring and organic matter and terrestrial material in summer, respectively. The fluxes of each chemical component observed with sediment traps are normalized to that of Al by assuming that the actual flux of Al is equal to the accumulation rate onto the sediment surface. Vertical changes of the normalized flux of each chemical component indicate the following: Fe was not regenerated from the settling particles in the water column. Mn was regenerated from the settling particles in the lower layer exclusively between 80 m depth and the sediment surface. Cd was actively regenerated in the upper layer above 80 m depth. Phosphate was regenerated in the upper layer, while biogenic silicate was in the lower layer. The silicate regeneration, therefore, occurs after phosphate regeneration. The material decomposing in the water column below 40 m has an atomic ratio of P ∶ Si ∶ C = 1 ∶ 52 ∶ 128. 相似文献
5.
Achieving long-term climate mitigation goals in Japan faces several challenges, starting with the uncertain nuclear power policy after the 2011 earthquake, the uncertain availability and progress of energy technologies, as well as energy security concerns in light of a high dependency on fuel imports. The combined weight of these challenges needs to be clarified in terms of the energy system and macroeconomic impacts. We applied a general equilibrium energy economic model to assess these impacts on an 80% emission reduction target by 2050 considering several alternative scenarios for nuclear power deployment, technology availability, end use energy efficiency, and the price of fossil fuels. We found that achieving the mitigation target was feasible for all scenarios, with considerable reductions in total energy consumption (39%–50%), higher shares of low-carbon sources (43%–72% compared to 15%), and larger shares of electricity in the final energy supply (51%–58% compared to 42%). The economic impacts of limiting nuclear power by 2050 (3.5% GDP loss) were small compared to the lack of carbon capture and storage (CCS) (6.4% GDP loss). Mitigation scenarios led to an improvement in energy security indicators (trade dependency and diversity of primary energy sources) even in the absence of nuclear power. Moreover, preliminary analysis indicates that expanding the range of renewable energy resources can lower the macroeconomic impacts of the long term target considerably, and thus further in depth analysis is needed on this aspect.
Key policy insights
For Japan, an emissions reduction target of 80% by 2050 is feasible without nuclear power or CCS.
The macroeconomic impact of such a 2050 target was largest without CCS, and smallest without nuclear power.
Energy security indicators improved in mitigation scenarios compared to the baseline.
6.
Molecular and isotopic characteristics of gas hydrate-bound hydrocarbons in southern and central Lake Baikal 总被引：4，自引：4，他引：0
Akihiro Hachikubo Oleg Khlystov Alexey Krylov Hirotoshi Sakagami Hirotsugu Minami Yutaka Nunokawa Satoshi Yamashita Nobuo Takahashi Hitoshi Shoji Shin’ya Nishio Masato Kida Takao Ebinuma Gennadiy Kalmychkov Jeffrey Poort 《Geo-Marine Letters》2010,30(3-4):321-329
We investigated the molecular composition (methane, ethane, and propane) and stable isotope composition (methane and ethane) of hydrate-bound gas in sediments of Lake Baikal. Hydrate-bearing sediment cores were retrieved from eight gas seep sites, located in the southern and central Baikal basins. Empirical classification of the methane stable isotopes (δ13C and δD) for all the seep sites indicated the dominant microbial origin of methane via methyl-type fermentation; however, a mixture of thermogenic and microbial gases resulted in relatively high methane δ13C signatures at two sites where ethane δ13C indicated a typical thermogenic origin. At one of the sites in the southern Baikal basin, we found gas hydrates of enclathrated microbial ethane in which 13C and deuterium were both highly depleted (mean δ13C and δD of –61.6‰ V-PDB and –285.4‰ V-SMOW, respectively). To the best of our knowledge, this is the first report of C2 δ13C–δD classification for hydrate-bound gas in either freshwater or marine environments. 相似文献
7.
S. Kida K. Niinuma S. Suzuki T. Tanaka R. Nakanura K. Takefuji N. Matsumura M. Kuniyoshi T. Daishido 《New Astronomy》2008,13(7):519-525
The Nasu Observatory, which is composed of eight 20 m elements, was constructed for observing radio transients over a wide field at 1400 MHz. We report on two radio transients detected in consecutive drift scanning observations at declination 32° over a period of about two months. One of the two transients, WJN J1039+3200, appeared at =10h39m40s±10s, δ=32°±0.4° on March 4, 2005, and the other one, WJN J0645+3200, appeared at =06h45m25s±10s, δ=32°±0.4° on March 24, 2005. Both exhibited flux densities in excess of 1 Jy, and the burst durations were up to two days. Since there are few examples of radio transients outside the Galactic plane, these are very important observations. We have previously reported on four radio transients with features that look like the two transients detected this time. Of these six WJN transients in total, five had a duration of up to two days, and one up to three days. Four of the transients were detected at high Galactic latitude of b > 30°. Counterparts of the six WJN transients included X-ray sources in four events and had a consistency of 66%. The consistency of γ-ray, PGC Galaxy, NVSS, and FIRST sources was concentrated at about 50%. We were not able to find any special features in the counterparts. The distribution was verified by making a log N–log S plot using data for the four previously detected transients and the new ones. As a result, the distribution of the radio transients that we observed might have an isotropic distribution not dependent on Galactic longitude and Galactic latitude. The detection probability was calculated based on the assumption of an isotropic distribution. The 2σ upper probability limit for detection of transients of 1000 mJy or more is 0.0049 [deg−2 yr−1]. We cannot yet identify these two radio transients, because their features are different from any radio bursts observed in the past. 相似文献
8.
Akihiro Hachikubo Oleg Khlystov Masato Kida Hirotoshi Sakagami Hirotsugu Minami Satoshi Yamashita Nobuo Takahashi Hitoshi Shoji Gennadiy Kalmychkov Jeffrey Poort 《Geo-Marine Letters》2012,32(5-6):419-426
This study reports measurements of the Raman spectra of Lake Baikal gas hydrates and estimations of the hydration number of methane-rich samples. The hydration number of gas hydrates retrieved from the southern Baikal Basin (crystallographic structure I) was approx. 6.1. Consistent with previous results, the Raman spectra of gas hydrates retrieved from the Kukuy K-2 mud volcano in the central Baikal Basin indicated the existence of crystallographic structures I and II. Measurements of the dissociation heat of Lake Baikal gas hydrates by calorimetry (from the decomposition of gas hydrates to gas and water), employing the hydration number, revealed values of 53.7–55.5?kJ?mol–1 for the southern basin samples (structure I), and of 54.3–55.5?kJ?mol–1 for the structure I hydrates and 62.8–64.2?kJ?mol–1 for the structure II hydrates from the Kukuy K-2 mud volcano. 相似文献
9.
Jeffrey Poort Oleg M. Khlystov Lieven Naudts Albert D. Duchkov Hitoshi Shoji Shin’ya Nishio Marc De Batist Akihiro Hachikubo Masato Kida Hirotsugu Minami Andrey Y. Manakov Marina V. Kulikova Alexey A. Krylov 《Geo-Marine Letters》2012,32(5-6):407-417
Thermal measurements and hydrate mapping in the vicinity of the K-2 mud volcano in Lake Baikal have revealed a particular type of association of thermal anomalies (29–121?mW?m–2) near hydrate-forming layers. Detailed coring within K-2 showed that hydrates are restricted to two distinct zones at sub-bottom depths exceeding 70–300?cm. Temperature data from stations with hydrate recovery and degassing features all display low thermal gradients. Otherwise, the thermal gradients within the mud volcano are generally increased. These findings imply a more complicated thermal regime than often assumed for mud volcanoes, with important roles for both fluids and hydrates. The coexistence of neighbouring low and high thermal anomalies is interpreted to result from discharging and recharging fluid activity, rather than hydrate thermodynamics. It is suggested that hydrates play a key role in controlling the fluid circulation pattern at an early stage. At a later stage, the inflow of undersaturated lake water would favour the dissolution of structure I hydrates and the formation of structure II hydrates, the latter having been observed on top of structure I hydrates in the K-2 mud volcano. 相似文献
10.
Shizuo Tsunogai Shinichiro Noriki Koh Harada Taro Kurosaki Yasunori Watanabe Masaru Maedaa 《Journal of Oceanography》1986,42(2):83-90
Settling particles were collected at 1,460 m and 3,760 m depth in the Antarctic Ocean with sediment traps of time series type. The total deployment period of 40 days was divided into four terms of 10 days each. Seawater samples were collected both at deployment and retrieval of the traps at each site. During the 42 days the concentration of silicate in the surface water decreased by 32%, whereas those of nitrate and phosphate decreased by only 4–5%. The total particulate flux in the Antarctic Ocean is the largest among those hitherto observed in the world ocean. The time variation of the particulate flux at 1,460 m depth almost coincided with that at 3,760 m. The settling particles were comprised roughly of 80% biogenic silica, 15% organic matter and 5% other substances including sea salt. The clay fraction was only 0.05% at 1,460 m depth. The settling flux of biogenic silica agrees fairly well with the calculated rate of change in the concentration of silicate in the surface 100 m. Thus it is concluded that preferential propagation of diatoms reduces the concentration of silicate prior to other nutrients in the Antarctic Ocean. 相似文献