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A membrane-discriminated gas phase analyzer is proposed for multicomponent determinations. Nitrogengas flows countercurrent through outer and inner channels in a tube-in-tube arrangement. The onlycommunication between the two channels occurs through a 500μm aperture covered by a porous PTFEmembrane. A mixture of organic compounds (up to four components) is injected into the inner channelby a heated backflushed injector and the sample components diffusing into the outer channel aremonitored by a flame ionization detector (FID). A calibration set, consisting of pure components, binary,ternary and quaternary mixtures (a total of 64 samples), provides the known data base: temporal profilesof the FID output as a function of sample composition, Although the overall response behavior is nota linearly additive function of individual analyte concentrations, the use of successive inverse multiplelinear regression (while continually altering the choice of the calibration samples considered for theforward regression, on the basis of the most recent values of the predicted unknown sample composition)is shown to yield analytical results for unknown samples that are in good agreement with their true values. 相似文献
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KEVIN ROBERT GURNEY RACHEL M. LAW A. SCOTT DENNING PETER J. RAYNER DAVID BAKER PHILIPPE BOUSQUET LORI BRUHWILER YU-HAN CHEN PHILIPPE CIAIS SONGMIAO FAN INEZ Y. FUNG MANUEL GLOOR MARTIN HEIMANN KAZ HIGUCHI JASMIN JOHN EVA KOWALCZYK TAKASHI MAKI SHAMIL MAKSYUTOV PHILIPPE PEYLIN MICHAEL PRATHER BERNARD C. PAK JORGE SARMIENTO SHOICHI TAGUCHI TARO TAKAHASHI CHIU-WAI YUEN 《Tellus. Series B, Chemical and physical meteorology》2003,55(2):555-579
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MELODY STEIN ANNIE ARNAUD‐VANNEAU THIERRY ADATTE DOMINIK FLEITMANN JORGE E. SPANGENBERG KARL B. FÖLLMI 《Sedimentology》2012,59(3):939-963
A major shift from Urgonian oligotrophic carbonate accumulation to orbitolinid‐rich mixed siliciclastic–carbonate deposition is observed near the Barremian–Aptian boundary in many sections both within and outside the shallow‐marine Tethyan Realm. This important facies change in the Swiss Helvetic Alps is documented here and interpreted in the context of general palaeoenvironmental change. To achieve this, a detailed micropalaeontological, sedimentological, mineralogical and geochemical study has been carried out on six sections across the upper part of the lower Schrattenkalk Member (Late Barremian), the Rawil Member (formerly ‘Lower Orbitolina Beds’, earliest Aptian) and the lowermost part of the upper Schrattenkalk Member (Early Aptian). The sediments of the Rawil Member exhibit inner‐platform facies with rudists, miliolids, orbitolinids and dasycladals to outer‐platform facies characterized by small benthic foraminifera, orbitolinids, crinoids and bryozoans. Stratigraphic trends in microfacies environments and the composition of microfossil assemblages, indicate that the Rawil Member includes a transgressive systems tract and the base of a highstand systems tract which are composed of an increasing number of parasequences in distal directions (five to nine in the sections studied here). The sea‐level rise discerned in the Rawil Member is coeval with increased detrital input and phosphorus burial, with maximum values up to 80 times and 21 times the background values in the subjacent part of the lower Schrattenkalk Member, respectively. Furthermore, the Rawil Member records the appearance of kaolinite, indicating a change towards tropical and more humid climate conditions. This change may have led to an increase in continental weathering rates and an associated increase in detrital and nutrient fluxes towards the ocean. The phase of climate change observed near the Barremian–Aptian boundary may have been triggered by a phase of intensified volcanic activity linked with the onset of the Ontong Java large igneous province and the Rawil Member may be the expression of a precursor episode to Oceanic Anoxic Event 1a in the shallow‐marine environment. 相似文献
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FAUSTO O. SARMIENTO 《Geographical review》2002,92(2):213-234
ABSTRACT. The anthropogenic nature of Andean ecosystems is discussed in the framework of tree‐line dynamics in selected sites in Ecuador. Indicators of human impact are evidence of the need for a scientific understanding of neotropical mountains that is better in tune with the special conditions of tropical Andean environments. Tropandean systems are neither tropical ecosystems nor midlatitude regions, and lessons from ecologically damaging activities in those ecosystems cannot be transferred readily to Tropandean systems. Better research from the ethnobiological and ecological fronts is needed if we are to comprehend the intricate functions of neotropical mountains, particularly the cloud‐forest belt, which is regarded as the most threatened ecosystem when considering sustainability scenarios. 相似文献
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FAUSTO O. SARMIENTO 《Geographical review》2010,100(2):229-245
The Andean lapwing (Vanellus resplendens Tschudi) prompts rethinking of ethnoecology in neotropical cloud forests and páramos and challenges notions about conservation in mountain protected areas. Using archaeological, historical, and current evidence, I argue that the role of humans in shaping viable high‐mountain bird populations is an important factor in the conservation priorities of tropandean landscapes, particularly in the mountains. The presence of the Andean lapwing demonstrates the intricate linkages between culture and nature in the Andean region. I highlight a paradox of conservation, using the Andean lapwing as the avian indicator of global environmental change as an example of the contest between landscape change, biodiversity, and ethnoecological insights. Landscape stewardship, conservation easements, and cultural landscapes are options for inclusion in the repertoire of scenarios for the survival of healthy avifaunal assemblages in high‐mountain environments that have evolved in synchrony with humans, such as in páramos, cultural landscapes worth protecting in the tropical Andes. 相似文献
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LAURA GALLARDO JORGE CARRASCO GUSTAVO OLIVARES 《Tellus. Series B, Chemical and physical meteorology》2000,52(1):50-59
Increases in tropospheric ozone (O3 ) abundance are likely to take place in the near future in the populous and rapidly developing countries in the tropics and subtropics. An accurate evaluation of the future impact of increasing industrial activities in tropical and subtropical areas requires knowledge of the background levels of ozone. New ozone monitoring stations have been installed at several sites by the World Meteorological Organization (WMO) since the mid‐90s. We analyze ozone data collected during two years since April 1996 at Cerro Tololo (30°S, 70°W, 2200 m.a.s.l.) some 50 km east from the city of La Serena. In this paper, we describe some of the atmospheric chemistry and meteorology that characterizes the Tololo site. The data show a seasonal variation with maximum mixing ratios in late winter and spring and minimum mixing ratios in late summer and early fall. These variations are most likely associated with the large‐scale subsidence of the Hadley circulation and the location of the subtropical jet stream (STJ). Also, there is a diurnal variation that is probably partly associated with a mountain wind flow which is strongest in late spring and summer months. No significant mixing with marine boundary layer air perturbed by anthropogenic activities is apparent from the data. We find the Cerro Tololo site to be generally representative for background conditions of free‐tropospheric air in the subtropics of the Southern Hemisphere. This work is done within the framework of a larger effort recently started by several Chilean institutions in cooperation with research centers abroad. 相似文献
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Sediment dynamics and hydrodynamics in the lower course of a river highly regulated by dams: the Ebro River 总被引：1，自引：0，他引：1
The lowest part of the Ebro River is a microtidal salt-wedge estuary. Penetration of the salt-wedge is largely controlled by the fluvial discharge and the morphology of the river bed, although sea level variations caused by tides and atmospheric conditions can also play significant roles. The concentration and distribution of suspended particulate matter in this part of the river and the fluvial sediment discharge are strongly influenced by the dynamics of the salt-wedge. Damming of the river has caused sediment to be trapped in reservoirs and has regulated the fluvial discharge. Intrusion of the salt wedge has thus also been regulated. At present, sediment discharge is between 1 and 1·5 × 105 tons per year, which is less than 1% of the sediment that the Ebro River discharged into the sea before construction of the dams. This extreme reduction in sediment supply has allowed marine erosional processes to dominate in the delta. 相似文献