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The task of identifying climatically significant regional anthropogenic emissions and estimating their contribution to the variability of nitrogen oxides observed at a monitoring station is considered on the basis of NO and NO2 surface concentrations measured at the Zotino background observation station (60°26′ N, 89°24′ E, Krasnoyarsk Territory). The approach used is based on an estimation of the conditional probability of polluted air arriving from individual regions by using the results of calculating backward Lagrangian trajectories in the lower troposphere. It is established that the contribution of air masses supplied from industrial regions in the south of the Krasnoyarsk Territory to episodes of high concentrations of nitrogen oxides (>0.7 ppb) is larger than the contribution from cities and towns located in the south of Western Siberia. The results indicate that anthropogenic sources of pollution substantially affect the balance of minor gases in the lower troposphere on a regional scale and that this factor must be taken into account when observational data from the Zotino background station are analyzed and interpreted.  相似文献   
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Analyzed are the results of meteorological and environmental measurements performed over the 60-year period (1954–2013) at the Meteorological Observatory of Lomonosov Moscow State University. The significant positive temperature trend (0.04°C/year for 1954–2013) was obtained; it increased up to 0.07°C/year in 1976–2012. Considered are the features of seasonal variations of different atmospheric characteristics. Discussed are the type and causes of low-frequency changes in meteorological parameters, radiation balance components, radiation in different spectral ranges, and chemical composition of precipitation. Demonstrated are possible mechanisms of the more significant increase observed in air temperature in Moscow as compared with that in Central Federal District and their connection with the greenhouse effect in the urban atmosphere.  相似文献   
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Doklady Earth Sciences - Estimates of the photochemical ozone generation rate, PQ, and the ozone production efficiency (OPE) per molecule of NOx (=NO + NO2), ∆P, are obtained for the region...  相似文献   
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Izvestiya, Atmospheric and Oceanic Physics - The results of an intensive complex experiment carried out from March 25 to May 3, 2020, to study the composition and time variability of urban aerosol...  相似文献   
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Izvestiya, Atmospheric and Oceanic Physics - Results obtained in the course of unique observations (as part of the TROICA project) of the composition and state of the atmosphere over Russia have...  相似文献   
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Pankratova  N. V.  Belikov  I. B.  Belousov  V. A.  Kopeikin  V. M.  Skorokhod  A. I.  Shtabkin  Yu. A.  Malafeev  G. V.  Flint  M. V. 《Oceanology》2020,60(5):593-602
Oceanology - In Russian Arctic seas, observations of surface methane concentrations (CH4), ozone, nitrogen and carbon oxides, as well as the content of $${{\delta...  相似文献   
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Izvestiya, Atmospheric and Oceanic Physics - This paper updates the results obtained earlier with the climate model developed at the A.M. Obukhov Institute of Atmospheric Physics of the Russian...  相似文献   
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A physically based cloud nucleation parameterization was introduced into an optical properties/radiative transfer module incorporated with the off-line air quality modeling system Regional Atmospheric Modeling System (RAMS)-Models-3 Community Multi Scale Air Quality (CMAQ) to investigate the distribution features of the first indirect radiative effects of sulfate, nitrate, and ammonium-sulfate-nitrate (ASN) over East Asia for the years of 2005, 2010, and 2013. The relationship between aerosol particles and cloud droplet number concentration could be properly described by this parameterization because the simulated cloud fraction and cloud liquid water path were generally reliable compared with Moderate Resolution Imaging Spectroradiometer (MODIS) retrieved data. Simulation results showed that the strong effect of indirect forcing was mainly concentrated in Southeast China, the East China Sea, the Yellow Sea, and the Sea of Japan. The highest indirect radiative forcing of ASN reached ?3.47 W m?2 over Southeast China and was obviously larger than the global mean of the indirect forcing of all anthropogenic aerosols. In addition, sulfate provided about half of the contribution to the ASN indirect forcing effect. However, the effect caused by nitrate was weak because the mass burden of nitrate was very low during summer, whereas the cloud fraction was the highest. The analysis indicated that even though the interannual variation of indirect forcing magnitude generally followed the trend of aerosol mass burden from 2005 to 2013, the cloud fraction was an important factor that determined the distribution pattern of indirect forcing. The heaviest aerosol loading in North China did not cause a strong radiative effect because of the low cloud fraction over this region.  相似文献   
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The results of experimental measurements of atmospheric methane concentrations and its isotopic composition in the Russian Arctic seas in the summer and autumn of 2015 are discussed. The Keeling plot method and inverse number simulation were used for revealing the factors responsible for elevated methane concentrations over the sea surface. Its maximum concentrations (up to 2050 ppb) were measured over the Kara and Laptev seas, as well as in the port area of Arkhangel’sk. It is shown that tundra and bog ecosystems of Siberia serve as the main sources of methane in the measurement zone (except for the area adjacent to large ports). As a whole, the share of methane from microbiological sources is as high as approximately 43% of the total methane concentrations along the ship route.  相似文献   
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