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1.
为揭示太湖流域降雨和湖水酸根阴离子长期变化特征及环境意义,通过历史数据收集和采样分析,对太湖流域降雨和湖水中的SO42-、NO3-变化特征和来源进行了研究.结果表明:自1990s以来太湖流域降雨中SO42-呈显著下降趋势,年平均下降率为0.28 mg/(L·a);NO3-浓度却呈显著上升趋势,年平均增长率为0.05 mg/(L·a),降雨中氮污染呈现加重的趋势.与之相反,湖水中SO42-呈显著上升趋势,年平均增长率为1.24 mg/(L·a);NO3-浓度却呈显著下降趋势,年平均下降率为0.02 mg/(L·a).30年以来,太湖水体SO42-/NO3-比值不断升高,远高于降水SO42-/NO3-比值.研究认为:流域SO2排放引起的酸沉降是湖水SO42-浓度增长的最重要原因,但氮氧化物排放并未引起湖水NO3-浓度升高,说明太湖流域对大气沉降的氮氧化物有滞留作用,而太湖水体是流域大气沉降硫酸盐的重要汇.综合治理太湖流域酸性物质排放对防止太湖水体酸化和治理富营养化都具有重要意义.  相似文献   

2.
在巢湖西北半湖近岸带设置大型围隔研究秋季连续打捞蓝藻对湖泊温室气体通量的影响,应用YL-1000型大型仿生式水面蓝藻清除设备进行原位打捞蓝藻,通过便携式温室气体分析仪-静态箱法对大型围隔内水-气界面CH4、CO2通量特征及其影响因素进行观测.结果表明:对比未打捞区,蓝藻连续打捞下打捞区水体中叶绿素a(Chl.a)、悬浮物(SS)浓度不断下降,两者削减率分别为72%、85%,Chl.a、SS浓度分别下降到29.6±2.5 μg/L、12.5±1.2 mg/L,打捞对围隔内颗粒态物质去除效果十分明显;打捞过程中水体溶解性有机物(DOM)中微生物代谢类腐殖质(C1)、类蛋白(C3)显著下降趋势,打捞区C1、C3组分(0.18±0.02、0.06±0.01 RU)强度明显低于未打捞区(0.26±0.05、0.12±0.03 RU),打捞能有效控制藻源性溶解性有机质释放.同时,打捞区水-气界面CH4通量呈显著下降趋势,未打捞区CH4通量平均值(17.473±1.514 nmol/(m2·s))为打捞区(7.004±4.163 nmol/(m2·s))近2倍,CH4通量与Chl.a、C1、C3组分均呈显著正相关,水体中藻源性溶解态有机质对CH4通量具有促进作用;打捞区CO2释放通量呈显著上升趋势,打捞区CO2吸收通量(-0.200±0.069 μmol/(m2·s))明显低于未打捞区(-0.344±0.017 μmol/(m2·s)),CO2通量与Chl.a、温度均呈显著负相关.秋季打捞对CH4、CO2综合日平均通量减排量值为0.275±0.076 mol/(m2·d)(以CO2当量计).研究结果揭示了巢湖秋季连续打捞蓝藻过程对水-气界面温室气体具有显著减排作用,且能在一定程度上减缓蓝藻水华与湖泊富营养化、气候变暖之间的恶性循环,为湖泊碳循环和蓝藻水华灾害防控提供科学数据支撑和理论参考.  相似文献   

3.
邓焕广  张智博  刘涛  殷山红  董杰  张菊  姚昕 《湖泊科学》2019,31(4):1055-1063
为了解城市湖泊不同水生植被区水体温室气体的溶存浓度及其影响因素,于2015年4-11月按每月2次的频率采用顶空平衡法对聊城市铃铛湖典型植被区——菹草区、莲藕区和睡莲区表层水中CO2、CH4和N2O的溶存浓度进行监测,计算水中温室气体的饱和度和排放通量,并测定水温(T)、pH、溶解氧(DO)、叶绿素a及营养盐浓度等理化指标,以探究水体环境因子对温室气体溶存浓度的影响.结果表明,铃铛湖各植被区水体温室气体均处于过饱和状态,是大气温室气体的"源";莲藕区CH4浓度、饱和度和排放通量均显著高于菹草区,而各植被区N2O和CO2均无显著性差异;不同植被区湖水中DO、总氮(TN)、总磷(TP)和硝态氮(NO3--N)浓度具有显著差异,其中DO、TN和NO3--N浓度均表现为菹草区最高,莲藕区最低,而TP浓度则正好相反;各植被区温室气体浓度和水环境参数间的相关分析和多元回归分析的结果表明,水生植物可通过影响水体的理化性质对温室气体的产生和排放产生显著差异影响,在菹草区亚硝态氮(NO2--N)、NO3--N、T和DO是控制水体温室气体浓度的主要因子;睡莲区为TP和pH;莲藕区则为pH、NO2--N和DO.  相似文献   

4.
我国快速的城镇化过程造成了河流氮、磷等营养盐的污染和潜在的水体富营养化问题.对城镇流域水体氮、磷污染特征及其演变趋势的识别具有重要意义.本研究选取长三角典型城镇地区宁波市北仑区小浃江流域为研究对象,在流域内根据空间分布、土地利用类型、人类活动强度等情况布设样点,于2017年夏季和冬季采集水样,研究流域水体氮、磷污染的时空分布特征并分析其污染来源和评估其富营养化水平.结果表明:流域内铵态氮(NH4+-N)、;硝态氮(NO3--N)、亚硝态氮(NO2--N)、总氮(TN)、总磷(TP)和叶绿素a(Chl.a)浓度范围分别为0.63~3.25 mg/L、0.52~3.75 mg/L、0.02~0.22 mg/L、1.61~12.86 mg/L、0.02~0.74 mg/L和0.6~60.57 μg/L.各个采样点氮、磷分布具有较大的空间异质性和季节变化规律.富营养化综合指数EI评估结果显示,整个流域富营养化程度属于贫至中营养级.氮、磷浓度与土地类型面积占比的Spearman相关性统计表明,100 m缓冲区建设用地面积占比与NH4+-N、NO2--N、TN、溶解氧(DO)浓度具有显著相关性,湿地面积占比与DO浓度呈显著正相关.汇水区域内林地面积占比与NH4+-N、NO2--N、TP、PO43--P、COD、Chl.a浓度呈显著负相关,与DO浓度呈显著正相关.相关性分析和冗余分析表明城镇化的面源污染及可能存在的点源污染是小浃江流域氮、磷污染的主要来源.因此,在小浃江流域100 m范围内,控制建设用地的规模和污染排放是减轻流域氮、磷污染的主要途径.在汇水区域内,增加林地植被的面积对减少氮、磷污染具有重要影响.  相似文献   

5.
通过模拟沙湖沉积物-水系统,以沙湖原水氟离子(F-)浓度为1倍浓度(0.69 mg/L),设置0.5倍浓度、1倍浓度、1倍浓度灭菌、2倍浓度和4倍浓度共5个实验组,探究不同上覆水F-浓度背景下沙湖沉积物中F-的迁移.结果表明,沉积物F-的释放量随上覆水F-浓度的增加而呈下降的趋势,其中2倍和4倍浓度组的沉积物由释放F-转变为吸附F-.碱性水体有利于沉积物F-的释放,即随着pH增大,F-释放量也会增加.微生物的Beta多样性层次聚类分析表明,F-会抑制PaenisporosarcinaThiobacillus的相对丰度,但对Fusibacter的生命活动具有促进作用.根据各浓度组间优势菌属相对丰度与环境因子的冗余分析可得,AcinetobacterThiobacillus相对丰度与pH呈负相关;Fusibacter相对丰度与F-浓度呈显著正相关,而Thiobacillus的相对丰度则与F-表现出弱负相关.通过对各浓度组中重要离子的分析发现,0.5倍组和4倍组中F-的迁移受Ca2+、HCO3-和SO42-浓度影响较大;相关性分析表明0.5倍浓度组的Ca2+、HCO3-浓度与F-浓度呈极显著正相关,而4倍组中F-浓度和Ca2+、HCO3-浓度呈负相关,SO42-浓度和F-浓度的相关性则是0.5倍组呈负相关,4倍组呈极显著正相关.本文在不同上覆水F-浓度背景下全面探究了沙湖沉积物中F-释放和迁移机理,为沙湖及其他含氟地表水的氟污染防治提供理论支持.  相似文献   

6.
崔旭  张兵  何明霞  夏文雪  王义东  赵勇 《湖泊科学》2021,33(6):1675-1686
生态补水是维持和改善白洋淀生态环境的重要途径.为研究生态补水对白洋淀水环境的影响,分别在补水前与补水后采集淀水、河水及地下水样品,分析区域地表水和地下水水化学特征.结果表明:(1)白洋淀补水前、后地表水与地下水的水化学组成中Na+为主要阳离子,补水后阴离子以HCO3-为主,淀区南部地表水电导率高;补水后地表水与地下水Ca2+、Mg2+和HCO3-浓度显著增加,水体电导率降低.(2)补水前地下水为Na-HCO3型水,地表水主要为Na-Cl·SO4及Na-Cl·HCO3类型;补水后地表水与浅层地下水向Ca·Mg-HCO3型演化,深层地下水水化学类型基本保持不变.(3)生态补水使白洋淀水位升高,淀区水面积增大,缓解了水资源短缺的问题;同时也使浅层地下水水化学组成发生改变,而深层地下水暂未受到影响.生态补水后,受稀释和混合作用的影响,水体Na+、Cl-和SO42-浓度显著下降,Ca2+、Mg2+及HCO3-浓度增加.在白洋淀生态补水中应"先治污,后补水",以减少补水过程中污染物向淀区的运移,还应注意区域地下水位上升过程中的阳离子交换及水岩相互作用,为合理调配生态补水及改善白洋淀生态环境提供科学依据.  相似文献   

7.
时历杰  王敏 《湖泊科学》2019,31(2):590-608
本文综合利用Na+,K+,Mg2+//Cl-,SO42--H2O五元体系干基图、水图、钠图,研究柴达木盆地一里坪盐湖硫酸盐型卤水水化学特征受外来淡水补给掺杂、选择性溶解、年温差等多因素影响产生的季节性变化,其中温度为主要因素.当卤水温度降低至0℃,开始析出芒硝,水化学变质系数MgSO4/MgCl2比值急剧下降,水化学特征由硫酸镁亚型向氯化物型转化过渡.通过20~25℃晶间卤水L10和L20蒸发实验研究,确定了一里坪卤水蒸发路线、液固相组成、物相鉴定、水化学特征系数、离子行为等变化及成盐特征,并与25℃ Na+,K+,Mg2+//Cl-,SO42--H2O五元体系介稳相图理论预测计算综合对比,二者吻合性比较好,整体相对误差能控制在5%范围内,利用相图理论计算能够很好地指导实际硫酸盐型卤水蒸发析盐.利用水化学特征系数KCl/MgCl2、MgSO4/MgCl2,研究了25℃硫酸盐型盐湖卤水钾盐成盐特征,当变质系数MgSO4/MgCl2高于0.13时,卤水钾盐矿物析出的同时,伴随有泻利盐共同析出.利用含Li+、borate、Mg2+水盐体系相图,研究一里坪老卤水深度蒸发中Li、B的行为,理论预测计算结果,剩余老卤水Mg2+/Li+比值降至27时,卤水中的Li、B始终以离子形式赋存于卤水中继续富集,此时卤水的累积成卤率仅为2.50%~3.20%,须引入新的工艺技术进行Li、B提取.研究结果为极高镁锂比、高镁硼比的硫酸盐型卤水的综合开发利用提供了理论支持.  相似文献   

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湖库淡水水域对温室气体排放的贡献不容小觑,然而观测时间的代表性不足以及缺乏对降雨因素的考虑制约了碳排放的准确估计.本研究以湖北宜昌境内官庄水库为例,选取强降雨多发的夏季时段,针对水气界面温室气体通量、水体表层和垂向剖面气体溶存浓度及环境因子开展了为期1周的原位高频观测,以探讨夏季降雨事件对水库温室气体通量变化的影响.结果表明,观测期内官庄水库水气界面CH4通量变化范围为0.007~0.077 mg/(m2·h),CO2通量范围为5.48~57.57 mg/(m2·h),白天和夜晚均表现为大气的碳源.小雨、中雨乃至暴雨天气条件下,CH4和CO2日均通量均较低,日通量倾向于受风速和温度调控.CH4和CO2通量变化趋势较为一致,观测期内日间排放量高于夜间排放量出现的次数更多,昼夜差异对降雨天气状况无明显响应,风速是CH4和CO2通量昼夜变化的主导因素.暴雨过程中,CH4-k600和CO2-k600与水气温差存在显著正相关,但水体垂向混合过程十分短暂.在平均雨强为3.8 mm/h的暴雨第I阶段,CH4-k600对风速和降雨的响应明显,而在雨强更大(8.5 mm/h)的第II阶段,CH4-k600与风速、降雨均未表现出相关性,通量箱在强降雨条件下的适用性可能存在雨强阈值.  相似文献   

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湖光岩玛珥湖水体中营养盐的时空分布特征及其影响因素   总被引:1,自引:0,他引:1  
湖光岩玛珥湖是世界上最大的玛珥湖,它几乎是封闭的,受外界的干扰小.目前有关玛珥湖的研究主要集中在古气候及生态环境研究方面,而有关玛珥湖营养盐在一年中的生物地球化学循环的研究较少,因此研究湖光岩玛珥湖营养盐的生物地球化学过程具有重要意义.于2015年10月-2016年9月对湖光岩玛珥湖全水柱的营养盐及其他相关参数进行逐月调查,分析营养盐的结构特征、垂直分布特征和时间变化情况,并讨论营养盐时空变化的影响因素.结果表明,湖光岩玛珥湖水中的无机氮(DIN)以铵态氮(NH4+-N)为主(>60%),其次是硝态氧(NO3--N),亚硝态氮(NO2--N)所占比利最低.湖光岩玛珥湖水中的硅酸盐(SiO32--Si)浓度较高,水体浮游植物生长受磷限制.冬季风期间,水体垂直混合较均匀,导致营养盐的垂直分布比较均匀;夏季风期间,水体层化,营养盐浓度在浅层水体较低,在深层水体较高.湖光岩玛珥湖表层水中的NO3--N、NH4+-N和SiO32--Si具有明显的时间变化规律:NO3--N浓度从10月-次年3月升高,从3-9月降低;NH4+-N浓度从10月-次年5月降低;SiO32--Si浓度从11月-次年5月降低,从5-9月持续升高.营养盐浓度的时间变化受有机质的矿化分解、水体的季节性混合、浮游植物的吸收、降雨的输入等多种因素的综合影响.  相似文献   

10.
水体甲烷(CH4)主要通过气泡和扩散传输排放到大气,这两种途径在CH4总排放中的相对贡献及环境影响因子目前关注较少.本文以洞庭湖湿地3种生境类型(光滩、苔草、芦苇)为研究对象,通过静态箱法和扩散模型法估算洪水期CH4总排放通量、扩散排放通量和气泡排放通量,并分析其水体环境因子影响.结果表明:苔草地CH4总排放量最高,为6.49±3.12 mg(C)/(m2·h).在3个生境中,CH4扩散排放占总排放通量的1.34%~3.91%,气泡排放占96.09%~98.66%.扩散排放通量受水体pH、电导率和水温的影响,而CH4的总排放和气泡排放主要受水温的影响.当水温低于11.7℃时,水体CH4以扩散排放为主,但当水温高于11.7℃时,水体CH4主要通过气泡排放.但这一温度阈值是否同样适用于其他类型湿地还需要更多实验验证.本研究对于揭示中低纬度内陆湖泊水体CH4排放过程有重要意义.  相似文献   

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正SCIENCE CHINA Earth Sciences,an academic journal cosponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China,and published by Science China Press and Springer,is committed to publishing high-quality,original results in both basic and applied research.  相似文献   

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正Director:Shangfu Kuang,China Vice-directors:Chunhong Hu,China Duihu Ning,China Guangquan Liu,China The International Research and Training Center on Erosion and Sedimentation(IRTCES)was jointly set up by the Government of China and UNESCO on July 21,1984.It aims at the promotion of international exchange of knowledge and cooperation in the studies of erosion and  相似文献   

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Feedback mechanisms, which operate upstream through drawdown and backwater effects and downstream through sediment discharge are responsible for channel evolution. By combining these mechanisms with channel processes it euables a dynamic process-response model to be developed to simulate the initial evolution of straight gravel-bed channels. When erosion commences on a land surface, sediment entrained in the headwater reach by hydraulic action is selectively transported, deposited and reworked. This produces a damped oscillation between degradation and aggradation as the channel and valley respond to spatial and temporal variations in sediment calibre and hydraulic conditions. The initial cut and fill phases are responsible for valley incision and floodplain development while secondary and subsequent activity can produce river terraces. Eventually sediment entrainment in the headwaters declines as slopes are reduced. Subsequent channel evolution is relatively insignificant because it is dependent on local weathering activity producing material that can be transported on declining slopes. Therefore landforms produced during the initial phase of development, when local weathering was non-limiting, dominate the landscape.  相似文献   

18.
Based on relocating the Jiujiang-Ruichang earthquake sequence which occurred on November 26, 2005 in Jiangxi Province with the double-difference (DD) algorithm and master event technique, the paper discusses the focal mechanism of the main shock (MsS.7) and the probable seismo-tectonics. The precise relocation results indicate that the average horizontal error is 0.31kin in a EW direction and 0.40kin in a NS direction, and the average depth error is 0.48kin. The focal depths vary from 8kin to 14kin, with the predominant distribution at 10kin - 12kin. The epicenter of the main shock is relocated to be 29.69^oN, 115.74^oE and the focal depth is about 10.Skin. Combining the predominant distribution of the earthquake sequence, the focal mechanism of the main shock and the tectonic conditions of N-E- and NW-strike faults growth in the seismic region, we infer that the main shock of the earthquake sequence was caused by a NW striking buried fault in the Rnichang basin. The nature of seismic faults needs to be further explored.  相似文献   

19.
Abstract

The western reservoirs represent the principal groundwater system in Morocco. Demographic, industrial and agricultural developments during the last decade have markedly altered groundwater quality. The Mamora coastal aquifer system is among the Atlantic systems which are most heavily threatened by pollution. Agricultural and industrial activities, and rapid urban growth contribute to the pollution of the groundwater. Contamination transport is facilitated by a high permeability of the aquifer formations. In order to assess the actual groundwater quality of the Mamora aquifer and to understand the influence of the factors generating the pollution, an extensive multidisciplinary research programme is in progress, with hydrochemistry and microbiology playing essential roles. The present paper concerns the spatial distribution of physico-chemical parameters in the groundwater, subjected to domestic, industrial and agricultural pollution. Fifty-seven samples were analysed for several parameters (Ca2+, Mg2+, Na+, K+, Cl?, SO4 2?, HCO3 ?, NO3 ?, pH, electrical conductivity and temperature). The microbiological analysis of 143 samples reveals the presence of four kinds of indicator bacteria in the groundwater resources: faecal Streptococci, faecal coliform, Escherichia coli and Clostridium. The physico-chemical results and bacteriological monitoring show that the nitrate and bacteria concentrations exceed the maximum admissible levels, notably around pumping stations in the sectors of Sidi Taibi, Sidi Ahmed Taleb and Aïn Sbaâ. Contamination is generated by uncontrolled anthropogenic activities and accentuated by the high intrinsic vulnerability of the aquifer system. Several parameters appeared to exceed admissibility standards. Measures are recommended to prevent groundwater pollution in the region.  相似文献   

20.
Zinc in the Environment. In 1990 the world production of zinc ammounted to 7 Mio. metric tons. The main areas of application were: galvanization, alloys like brass and zinc metal. The content in the earth crust varies between 10–300 ppm zinc with a mean of 70 ppm. Uncontaminated surface waters contain less than 10 mg/m3 zinc. Apart from civilization air contains 1–10 ng zinc per m3. These background concentrations are exceeded by orders of magnitude in zinc deposit areas and where anthropogenic influences predominate. Accumulation can occur in sediments and sewage sludge. Molluscs and Algae also accumulate zinc. Zinc is essential for live. With normal food the zinc supply of man is just sufficient. Bioaccumulation of zinc towards man or chronic oversupply of man is not known. Zinc has no teratogenic or mutagenic effects, a suspicion on a carcinogenic effect proved wrong. In stockbreeding and plant cultivation a minimum supply of zinc is necessary. Plants are relatively less sensitive against higher soil contents of zinc. Considering the toxicological and ecotoxicological effects of zinc in the environment, the critical organismens are marine invertebratae like tubifex, daphnia, gammarus and algae. But normally only a minor part of the total zinc contest is biologically available, depending on salt content and pH of the waters.  相似文献   

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