共查询到18条相似文献，搜索用时 296 毫秒
1.
《中国地理与资源文摘》2005,(1)
X13,X14 4 2 0 0 5 0 10 0 6 6长江口潮滩有机质来源的C、N稳定同位素示踪 =CarbonandnitrogenstableisotopesastracerstosourceorganicmatterintheYangtzeEstuary/刘敏 ,侯立军…∥地理学报 .—2 0 0 4 ,5 9(6 ) .— 918～ 92 6依据长江河口潮滩自然环境特征和受人文活动影响的差异性 ,沿长江河口南岸潮滩选取了 12个典型的监测站位 ,并分别于洪水季节 (7月份 )和枯水季节 (2月份 )在各监测站位进行了表层 (0 - 2cm)沉积物样品的采集 .对表层沉积物有机质中稳定碳、氮同位素进行分析与测试发现 ,7月份稳定碳同位素值普遍低于 2月份的稳… 相似文献
2.
长江口潮滩有机质稳定碳同位素时空分布与来源分析 总被引：5，自引：0，他引：5
通过测定长江口潮滩悬浮颗粒有机质和表层沉积有机质在枯水季节 (2006年2月 )和洪水季节 (2006年8月 )的稳定碳同位素值,对有机质潜在来源及局部岸段改造作用进行了分析。结果显示,悬浮颗粒有机质稳定碳同位素值在2月明显低于8月,变化范围分别在-25.8‰~-23.4‰和-25.1‰~-22.9‰,主要是受径流量枯洪季变化和浮游生物生长季节变化两种因素的叠加作用。表层沉积有机质2月和8月的稳定碳同位素分别为-25.0‰~-20.4‰和-24.7‰~-19.5‰,季节变化不明显,主要来自悬浮颗粒物的沉降。除受大背景环境因素影响,局部环境对潮滩有机质也有一定的改造作用,污水、支流河水的输入对悬浮颗粒有机质碳同位素有一定的影响,埋藏的潮滩植物和底栖微藻则对沉积有机质有部分贡献。 相似文献
3.
西江河口段溶解无机碳稳定同位素组成的时空变化 总被引：2，自引：0，他引：2
从2006 年9 月至2007 年6 月间对西江河口段溶解无机碳稳定同位素组成(δ13CDIC) 及 其相关的水体理化参数进行了一个水文年的季节性采样调查。夏、秋两季δ13CDIC 平均值(-13. 91‰、-13.09‰) 小于春、冬季节(-11.71‰、-12.26‰), 呈现出明显的季节性。δ13CDIC 与温度 呈负相关(p = 0.000; r = -0.646), 而与氧化还原电位正相关(p = 0.000; r = 0.569), 表明河段 表层水体δ13CDIC 受到季节性变化的水体理化性质等河道有机质氧化分解条件的控制; 夏季洪水期δ13CDIC 与航测距离呈正相关, 而春季枯水期的δ13CDIC 与航测距离负相关。δ13CDIC 的这种时空变异证明了研究河段河- 海作用过程影响了水体的理化性状进而控制了河道表层水体DIC 的性质。研究河段δ13CDIC 的上述时空分布规律与流域所处的地理环境关系密切, 汛期的夏季受陆源有机质的强烈分解作用的影响, DIC 的同位素组成向海洋方向变轻; 枯期的春季因海洋作用加强以及咸潮的入侵, 河道DIC 的同位素组成向海洋方向变重。 相似文献
4.
长江口外海域沉积物中有机物的来源及分布 总被引：10，自引：0，他引：10
通过分析长江口外海域不同区域有机碳和氮的分布特征及其影响因素,了解了底部沉 积物中有机碳和氮同位素的生物地球化学特征,探讨二者对长江口外海域底部沉积物中有机 物来源的指示意义。运用质量混合模型,计算了长江输入的陆源有机物的贡献及其空间变化。结果表明,长江口外海域沉积物中TOC 和TN 的分布和东海陆架的环流体系有着密切关系, 与环流的分布相对应,如果大致沿31oN 和123oE 作为分界线, 整个研究区的TOC 和TN 的分布可划分为4 个具有不同分布特征的区域。TOC、TN、δ13C 和δ15N 分别与沉积物的平均粒 径呈线性相关关系,因此,粒度效应是控制长江口外海域沉积物中有机物分布和稳定同位素 碳、氮的一个重要因素。研究区内的C/N 比值能够在一定程度上体现有机物的来源信息,但δ15N 表现出了与C/N 和δ13C 不同的区域分布和变化特征。陆源有机物来源比重较高的区域与 长江口外海域赤潮突发频率最高的地区相对应。长江口附近沉积物中的陆源有机物来源最高, 超过了50%,且等值线呈舌状向东北方向凸出,表明了长江冲淡水的影响。陆源颗粒态有机物沉海底后,要不断经历早期成岩作用和生物作用,因此在在相同地点,陆源有机物对沉积物中有机物的贡献,要明显小于对悬浮颗粒态有机物的贡献。 相似文献
5.
对研究区内第五次北极科学考察所取的表层海水颗粒物的浓度、显微组成、有机碳、氮含量及其同位素组成进行了分析。结果表明,楚科奇海域表层海水颗粒物浓度介于0.56—4.01 mg·L-1,具有冰区边缘高于开阔水域的特点。陆架区颗粒有机质相对含量高(TOC:9.78%—20.24%;TN:0.91%—2.31%),有机碳、氮同位素值相对重(δ13C:-23.29‰—-26.33‰PDB;δ15N:6.14‰—7.78‰),有机质主要来源于海洋生物,含有部分陆源有机质;陆坡及北冰洋核心区的颗粒有机质含量,除SR15站外,相对低(TOC:8.06%—8.96%;TN:0.46%—0.72%),有机碳、氮同位素值轻(δ13C:-26.93‰—-27.78‰PDB;δ15N:4.13‰—4.84‰),颗粒物有机质以陆源为主。陆坡区SR15站表层海水颗粒物中异常高的陆源有机质(TOC:27.94%,TN:1.16%;δ13C:-27.43;δ15N:3.81)可能来自源于东西伯利亚的穿极洋流。海冰携带的颗粒物(包括冰藻)是冰区边缘表层海水颗粒物的重要来源,在陆架区海冰融化,向水体中释放了大量生物体;而陆坡区和北冰洋核心区,海冰对颗粒物的贡献以碎屑矿物和黏土矿物为主。 相似文献
6.
长江口拦门沙河段潮滩表层沉积物分布特征 总被引：4，自引：1，他引：3
基于2005年7月及2007年5月在长江订拦门沙河段崇明东滩、横沙东滩(浅滩)、九段沙以及南汇边滩等四大潮滩的水下滩地采集的大面积、高密度表层沉积物以及实测水文资料,对拦门沙河段潮滩表层沉积物颗粒度、参数、组成、类型以及分布特征进行分析,并在此基础上探讨影响沉积物分布的主要动力因子.结果表明:长江河口四大潮滩表层沉积物主要由砂、粉砂质砂和粘土质粉砂三种类型组成.沉积物中值粒径分布比较复杂,介于2.5～8ψ之间;沉积物分选系数集中于1～2左右,其分布与中值粒径具有一致性,其中物质组成相对较粗的颗粒分选性较好而较细的颗粒分选性较差:偏态与峰态跨度较大,分别介于0.1-0.8与1-4不等.崇明东滩、横沙东滩(浅滩)和九段沙的沉积物分选系数、偏态和峰态的分布具有一致性,三者相关性较强;南汇边滩的沉积物分选性、偏态及峰态值则因南滩与东滩所处位置差异而有较大差别.此外,河口潮滩表层沉积物分布显示泥沙输移的结果,其主要水动力因子包括潮流和波浪控制的泥沙输移:在受落潮优势流作用的地区普遍粗于涨潮优势流作用的地区;在波浪动力强、波能释放的地区沉积物普遍较粗且分选性较好:深水航道工程的堵汉、导流、破水波作用明显,使得导堤两侧的表层沉积物粒度出现粗细分布不均的特点. 相似文献
7.
滇池流域宝象河水库沉积物中有机碳的来源 总被引：1，自引：0，他引：1
通过对滇池流域宝象河水库沉积物TOC、TN、C/N、δ13C及粒度等指标的测定,分析了沉积物中有机碳的主要来源及其变化趋势。结果表明:水体中不同位置沉积物有机碳来源并不相同,距三岔河入库河口相对较近的沉积柱芯A中C/N比值介于2.93~11.73,δ13C值介于-23.66‰~-21.78‰,有机碳主要来源于水生生物,陆源输入贡献较小,有机碳含量受粒径大小影响显著;距三岔河入库河口相对较远的沉积柱芯B中,其TOC和TN含量较高,分别介于14.62~24.93 g?kg-1和2.11~3.3 g?kg-1,δ13C值变化范围为-28.36‰~-26.36‰,粒度以黏土和细粉砂为主,有机碳主要来源于水库周边陆源输入,受人类活动影响强烈。 相似文献
8.
沿海不同年限围垦区土壤剖面有机碳同位素与粒度特征——以江苏省东台市为例 总被引：1，自引：1，他引：0
根据江苏沿海不同年限围垦区土壤剖面有机碳稳定同位素(δ13C)与粒度资料,研究了不同年限围垦区土壤粒度特征变化情况与有机质来源变化特征。结果表明,在气候和母质基本相同的条件下,土壤δ13C和粒度特征主要受围垦年限和人类活动干扰影响。随着围垦年限的增加,土壤平均粒径显著降低,表现为DT7(33.93μm,林地,已围垦近60 a)DT1(46.10μm,农用地,已围垦16 a)DT6[48.21μm,盐蒿(Suaeda salsa)滩,已围垦2 a]。其中,DT6、DT7(30 cm以下)、DT1剖面粒度记录均具有自下向上逐渐变细的特点,粗颗粒组分逐渐减少,反映了粉砂淤泥质海岸围垦前原始潮滩沉积物的自然演化特点,DT7剖面30 cm以上逐渐变粗则可能主要由于已围垦近60 a里表层堆积了大量枯枝落叶所致。人类活动干扰在沉积记录中也较明显,DT6盐蒿滩剖面δ13C值总体上表现为海洋自生有机碳,主要反映原始沉积母质特征。DT1农用地剖面0~40 cm耕作层由于受开垦、翻耕、除草、施肥等各种人类活动干扰较大,各粒度组成及粒度参数均开始出现显著变化,这在表层迅速变轻的δ13C值也有所反映。DT7林地剖面尽管受人类干扰相对较小,但由于受到表层堆积的大量枯枝落叶等凋落物的影响,各粒度组成及参数在上部均也表现出明显变化,特别是表层0~10 cmδ13C值已呈明显的陆源性。δ13C值所表现出的陆源和海洋自生有机碳特征与根据经验公式计算的结果也具有较好的一致性。 相似文献
9.
为了了解扎龙湿地克钦湖沉积物中营养物质的分布状况,在扎龙湿地克钦湖设置了21个采样点,于2016年7月9日,采集了0~5 cm深度的沉积物样品,测定了表层沉积物样品中有机质、全氮和全磷含量;利用克里金插值法,绘制表层沉积物有机质、全氮和全磷含量的空间分布图,并分析了其空间分布特征及影响因素。研究结果表明,克钦湖0~5 cm深度沉积物中有机质和全磷含量整体上由东北向西南逐渐减小,北湖区表层沉积物中的有机质和全磷含量都大于南湖区;克钦湖中西部表层沉积物中的全氮含量较大,东南部的较小,南、北湖区表层沉积物中全氮含量平均值较接近;克钦湖表层沉积物整体呈弱碱性,北湖区表层沉积物组成以粉砂土为主,南湖区表层沉积物组成以砂土为主;表层沉积物中有机质、全氮和全磷含量与研究区的地势、植物群落分布和周边人类活动有关,粉砂土含量和pH是影响表层沉积物中有机质、全氮和全磷含量分布的主要指标。 相似文献
10.
阜康典型荒漠C3植物稳定碳同位素值的环境分析 总被引：26，自引：3，他引：23
通过对阜康典型荒漠C3植物稳定碳同位素值的分析。叶片炭同位素值在-23‰和-29‰之间变化,其中主要在-27‰附近波动。这与前人报道的世界上其他地区荒漠植物碳同位素值的变化非常一致。降水可以改变叶片碳同位素值的大小,降水越多,叶片碳同位素值越负,它们的变化幅度有物种的依赖性。叶片碳同位素值也受植物生长形式或期望寿命的影响,木本植物或寿命长的植物叶片碳同位素值要高。分析表明,利用该区土壤或陆相沉积中有机质碳同位素值可以判断气候的干湿变化：土壤或陆相沉积中有机质碳同位素值越高,气候则越干燥。 相似文献
11.
The spatial distribution patterns of total organic carbon and total nitrogen show significant correlations with currents of the East China Sea Shelf. Corresponding to distribu-tions of these currents, the study area could be divided into four different parts. Total organic carbon, total nitrogen, and organic carbon and nitrogen stable isotopes in sediments show linear correlations with mean grain size, respectively, thus “grain size effect” is an important factor that influences their distributions. C/N ratios can reflect source information of organic matter to a certain degree. In contrast, nitrogen stable isotope shows different spatial distri-bution patterns with C/N and organic carbon stable isotope, according to their relationships and regional distributions. The highest contribution (up to 50%) of terrestrial organic carbon appears near the Changjiang Estuary with isolines projecting towards northeast, indicating the influence of the Changjiang dilution water. Terrestrial particulate organic matter suffers from effects of diagenesis, benthos and incessant inputting of dead organic matter of plankton, after depositing in seabed. Therefore, the contribution of terrestrial organic carbon to par-ticulate organic matter is obviously greater than that to organic matter in sediments in the same place. 相似文献
12.
长江口外海域沉积物中有机物的来源及分布 总被引：1，自引：1，他引：0
The spatial distribution patterns of total organic carbon and total nitrogen show significant correlations with currents of the East China Sea Shelf. Corresponding to distributions of these currents, the study area could be divided into four different parts. Total organic carbon, total nitrogen, and organic carbon and nitrogen stable isotopes in sediments show linear correlations with mean grain size, respectively, thus ＂grain size effect＂ is an important factor that influences their distributions. C/N ratios can reflect source information of organic matter to a certain degree. In contrast, nitrogen stable isotope shows different spatial distribution patterns with C/N and organic carbon stable isotope, according to their relationships and regional distributions. The highest contribution （up to 50%） of terrestrial organic carbon appears near the Changjiang Estuary with isolines projecting towards northeast, indicating the influence of the Changjiang dilution water. Terrestrial particulate organic matter suffers from effects of diagenesis, benthos and incessant inputting of dead organic matter of plankton, after depositing in seabed. Therefore, the contribution of terrestrial organic carbon to particulate organic matter is obviously greater than that to organic matter in sediments in the same place. 相似文献
13.
长江口盐沼土壤有机质更新特征的滩面趋势 总被引：1，自引：0，他引：1
Characteristics and tidal flat trends of soil organic matter （SOM） turnover were studied for the Chongmingdongtan Salt Marsh in the Yangtze River estuary, based on analyses of stable carbon isotope composition （δ^13C）, grain sizes and contents of particulate organic carbon （POC）, total nitrogen （TN） and inorganic carbon （TIC） for three cores excavated from high tidal flat, middle tidal flat and bare flat. Results demonstrate that correlations between soil POC contents and δ^13C values of the salt marsh cores were similar to those between soil organic carbon （SOC） contents and δ^13C values of the upper soil layers of mountainous soil profiles with different altitudes. SOM of salt marsh was generally younger than 100 years, and originated mainly from topsoil erosions in catchments of the Yangtze River. Correlations of TN content with C/N ratio, POC content with TIC content and POC content with δ^13C values for the cores suggest that turnover degrees of SOM from the salt marsh are overall low, and trends of SOM turnover are clear from the bare flat to the high tidal flat. Bare flat samples show characteristics of original sediments, with minor SOM turnover. Turnover processes of SOM have occurred and are discernable in the high and middle tidal flats, and the mixing degrees of SOM compartments with different turnover rates increase with evolution of the muddy tidal flat. The exclusive strata structure of alternate muddy laminae and silty laminae originated from dynamic depositional processes on muddy tidal flat was a great obstacle to vertical migration of dissolved materials, and SOM turnover was then constrained. The muddy tidal flat processes exerted direct influences on sequestration and turnover of SOM in the salt marsh, and had great constraints on the spatial and temporal characteristics of SOM turnover of the Chongmingdongtan Salt Marsh in the Yangtze River estuary. 相似文献
14.
西南地区大气降水中氢氧稳定同位素特征与水汽来源 总被引：8，自引：0，他引：8
为阐明西南地区稳定同位素与大气降水的关系,对GNIP昆明、贵阳、桂林、成都站点δD和δ18O进行分析,初步建立当地大气降水线方程,并与中国及全国降水线方程进行对比,揭示该降水线方程的特征.研究表明：大气降水稳定同位素组成受到温度、蒸发、水汽源地等多种因素的相互影响,在不同时间有很大差异.西南地区降水中的δ18O值表现出“夏高冬低”的季节特点.d值呈现出降水中过量氘水汽来源不同的特点,贵阳和桂林地区d值表现为“冬高夏低”的季节特点,而昆明和成都地区却与此相反,d值则表现为“夏高冬低”独特的季节性特征. 相似文献
15.
长江口盐沼土壤有机质更新特征的滩面趋势 总被引：9，自引：0，他引：9
通过对长江口崇明东滩高潮滩、中潮滩以及光滩柱状样的有机元素(C、N)含量与碳稳定同位素组成(δ13C)、粒度组成等的测定,研究盐沼土壤有机质更新特征及其滩面趋势.结果表明,长江口盐沼土壤POC-δ13C相关特征与山地土壤剖面上部土层的基本类似,盐沼土壤有机质主要源于长江流域表层土壤,有机质年龄不足100年.不同高程柱样TN-C/N、POC-TIC与POC-δ13C关系特征表明盐沼土壤有机质更新程度普遍较低,有机质更新特征呈明显的滩面变化趋势.光滩有机质基本反映沉积母质特征,更新程度极低;中、高潮滩有机质更新作用已经发生,随着滩面演变,处于不同更新阶段的有机质组分混杂程度提高.盐沼滩面过程塑造垂向沉积层序,层序中独特的沙、泥纹层构造导致物质上下运移困难,有机质更新作用受到抑制.盐沼滩面过程直接影响有机质的累积与更新,对于有机质更新的时空特征具有显著制约. 相似文献
16.
基于多参数指标的长江口滨岸多环芳烃来源辨析 总被引：2，自引：0，他引：2
在长江口滨岸及临近排污口、滨岸河流、城市中心城区采集悬浮颗粒物、表层沉积物、街道灰尘等样品, 分别利用GC-MS 和GC-C-IRMS 定量分析了不同环境介质中的多环芳烃 (PAHs) 与有机单体化合物稳定碳同位素(δ13C), 开展了基于PAH 环数、分子量特征比值和有机单体化合物稳定碳同位素组成等参数指标的长江口滨岸悬浮颗粒物与表层沉积物中PAHs 源解析研究。研究结果显示, 长江口滨岸悬浮颗粒物与表层沉积物中的PAH 化合物主要以3~4 环为主, 与吴淞排污口、石洞口污水处理厂、黄浦江、滨岸小河流以及上海中心城区等潜在来源区域不同环境介质中的PAHs 组成特征相似, 主要来源于汽油、柴油、煤炭和木材的不完全燃烧以及石油残余物的混合。其中, 木材和煤炭不完全燃烧形成的PAHs 以及石油残余物, 枯季经过滨岸河流及排污口直接输入, 洪季则为城市街道灰尘被暴雨冲刷, 随地表 径流最终汇入河口; 汽车排放(汽油、柴油不完全燃烧) 产生的PAHs 主要富集在城市交通区和商业区的街道灰尘中, 枯季借助区域盛行风迁移至河口区, 洪季则主要通过暴雨径流冲刷进入河口。 相似文献
17.
Samples of suspended particulate matters (SPMs), surface sediment and road dust were collected from the Yangtze estuarine and nearby coastal areas, coastal rivers, and central Shanghai. The samples were analyzed for the presence of 16 polycyclic aromatic hydrocarbons (PAHs) in the USEPA priority-controlled list by GC-MS. The compound-specific stable carbon isotopes of the individual PAHs were also analyzed by GC-C-IRMS. The sources of PAHs in the SPMs and surface sediments in the Yangtze estuarine and nearby coastal areas were then identified using multiple source identification techniques that integrated molecular mass indices with organic compound-specific stable isotopes. The results revealed that 3-ring and 4-ring PAH compounds were dominant in the SPMs and surface sediments, which are similar to the PAH compounds found in samples from the Wusong sewage discharge outlet, Shidongkou sewage disposal plant, Huangpu River, coastal rivers and central Shanghai. Principal component analysis (PCA) integrated with molecular mass indices indicated that gasoline, diesel, coal and wood combustion and petroleum-derived residues were the main sources of PAHs in the Yangtze Estuary. The use of PAH compound- specific stable isotopes also enabled identification of the PAHs input pathways. PAHs derived from wood and coal combustion and petroleum-derived residues were input into the Yangtze Estuary and nearby coastal areas by coastal rivers, sewage discharge outlets during the dry season and urban storm water runoff during the flood season. PAHs derived from vehicle emissions primarily accumulated in road dust from urban traffic lines and the commercial district and then entered the coastal area via the northwest prevailing winds in the dry season and storm water runoff during flood season. 相似文献
18.
Jennifer L. Mays Mark Brenner Jason H. Curtis Kathryn V. Curtis David A. Hodell Alex Correa-Metrio Jaime Escobar Andrea L. Dutton Andrew R. Zimmerman Thomas P. Guilderson 《Journal of Paleolimnology》2017,57(4):307-319
Sediment core PI-6 from Lake Petén Itzá, Guatemala, possesses an ~85-ka record of climate and environmental change from lowland Central America. Variations in sediment lithology suggest large and abrupt changes in precipitation during the last glacial and deglacial periods, and into the early Holocene. We measured stable carbon isotope ratios of total organic carbon and long-chain n-alkanes from the core, the latter representing a largely allochthonous (terrestrial) source of organic matter, to reveal past shifts in the relative proportion of C3–C4 terrestrial biomass. We sought to test whether stable carbon isotope results were consistent with other paleoclimate proxies measured in the PI-6 core, and if extraction and isotope analysis of n-alkanes is warranted. The largest δ13C variations are associated with Heinrich Events. Carbon isotope values in sediments deposited during the last glacial maximum indicate moderate precipitation with little fluctuation. The deglacial was a period of pronounced climate variability, e.g. a relatively warm and moist Bølling–Allerød, but a cool and dry Younger Dryas. Arid periods of the deglacial were inferred from samples with high δ13C values in total organic carbon, which reflect times of greater proportions of C4 plants. These inferences are supported by stable isotope measurements on ostracod shells and relative abundance of grass pollen from the same depths in core PI-6. Similar trends in carbon stable isotopes measured on bulk organic carbon and n-alkanes suggest that carbon isotope measures on bulk organic carbon in sediments from this lake are sufficient to infer past climate-driven shifts in local vegetation. 相似文献