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1.
The source and hydrochemical makeup of a stream reflects the connectivity between rainfall, groundwater, the stream, and is reflected to water quantity and quality of the catchment. However, in a semi-arid, thick, loess covered catchment, temporal variation of stream source and event associated behaviours are lesser known. Thus, the isotopic and chemical hydrographs in a widely distributed, deep loess, semi-arid catchment of the northern Chinese Loess Plateau were characterized to determine the source and hydrochemical behaviours of the stream during intra-rainfall events. Rainfall and streamflow were sampled during six hydrologic events coupled with measurements of stream baseflow and groundwater. The deuterium isotope (2H), major ions (Cl, SO42−, NO3, Ca2+, K+, Mg2+, and Na+) were evaluated in water samples obtained during rainfall events. Temporal variation of 2H and Cl measured in the groundwater and stream baseflow prior to rainfall was similar; however, the isotope compositions of the streamflow fluctuated significantly and responded quickly to rainfall events, likely due to an infiltration excess, overland dominated surface runoff during torrential rainfall events. Time source separation using 2H demonstrated greater than 72% on average, the stream composition was event water during torrential rainfall events, with the proportion increasing with rainfall intensity. Solutes concentrations in the stream had loglinear relationships with stream discharge, with an outling anomaly with an example of an intra-rainfall event on Oct. 24, 2015. Stream Cl behaved nonconservative during rainfall events, temporal variation of Cl indicated a flush and washout at the onset of small rainfall events, a dilution but still high concentration pattern in high discharge and old water dominated in regression flow period. This study indicates rainfall intensity affects runoff responses in a semi-arid catchment, and the stored water in the thick, loess covered areas was less connected with stream runoff. Solute transport may threaten water quality in the area, requiring further analysis of the performance of the eco-restoration project.  相似文献   
2.
Redox hot spots occurring as metal-rich anoxic groundwater discharges through oxic wetland and river sediments commonly result in the formation of iron (Fe) oxide precipitates. These redox-sensitive precipitates influence the release of nutrients and metals to surface water and can act as ‘contaminant sponges’ by absorbing toxic compounds. We explore the feasibility of a non-invasive, high-resolution magnetic susceptibility (MS) technique to efficiently map the spatial variations of magnetic Fe oxide precipitates in the shallow bed of three rivers impacted by anoxic groundwater discharge. Laboratory analyses on Mashpee River (MA, USA) sediments demonstrate the sensitivity of MS to sediment Fe concentrations. Field surveys in the Mashpee and Quashnet rivers (MA, USA) reveal several discrete high MS zones, which are associated with likely anoxic groundwater discharge as evaluated by riverbed temperature, vertical head gradient, and groundwater chemistry measurements. In the East River (CO, USA), widespread cobbles/rocks exhibit high background MS from geological ferrimagnetic minerals, thereby obscuring the relatively small enhancement of MS from groundwater induced Fe oxide precipitates. Our study suggests that, in settings with low geological sources of magnetic minerals such as lowland rivers and wetlands, MS may serve as a complementary tool to temperature methods for efficiently mapping Fe oxide accumulation zones due to anoxic groundwater discharges that may function as biogeochemical hot spots and water quality control points in gaining systems.  相似文献   
3.
When the observation of small headwater catchments in the pre-Alpine Alptal valley (central Switzerland) started in the late 1960s, the researchers were mainly interested in questions related to floods and forest management. Investigations of geomorphological processes in the steep torrent channels followed in the 1980s, along with detailed observations of biogeochemical and ecohydrological processes in individual forest stands. More recently, research in the Alptal has addressed the impacts of climate change on water supply and runoff generation. In this article, we describe, for the first time, the evolution of catchment research at Alptal, and present new analyses of long-term trends and short-term hydrologic behaviour. Hydrometeorological time series from the past 50 years show substantial interannual variability, but only minimal long-term trends, except for the ~2°C increase in mean annual air temperature over the 50-year period, and a corresponding shift towards earlier snowmelt. Similar to previous studies in larger Alpine catchments, the decadal variations in mean annual runoff in Alptal's small research catchments reflect the long-term variability in annual precipitation. In the Alptal valley, the most evident hydrological trends were observed in late spring and are related to the substantial change in the duration of the snow cover. Streamflow and water quality are highly variable within and between hydrological events, suggesting rapid shifts in flow pathways and mixing, as well as changing connectivity of runoff-generating areas. This overview illustrates how catchment research in the Alptal has evolved in response to changing societal concerns and emerging scientific questions.  相似文献   
4.
Numerous efforts have been made to understand stemflow dynamics under different types of vegetation at the inter-event scale, but few studies have explored the stemflow characteristics and corresponding influencing factors at the intra-event scale. An in-depth investigation of the inter- and intra-event dynamics of stemflow is important for understanding the ecohydrological processes in forest ecosystems. In this study, stemflow volume (FV), stemflow funnelling ratio (FR), and stemflow ratio (F%) from Quercus acutissima and Broussonetia papyrifera trees were measured at both inter- and intra-event scales in a subtropical deciduous forest, and the driving factors, including tree species and meteorological factors were further explored. Specifically, the FV, FR and F% of Q. acutissima (52.3 L, 47.2, 9.6%) were lower than those of B. papyrifera (85.1 L, 91.2, 12.4%). The effect of tree species on FV and F% was more obvious under low intensity rainfall types. At the inter-event scale, FV had a strong positive linear correlation with rainfall amount (GP) and event duration (DE) for both tree species, whereas FR and F% had a positive logarithmic correlation with GP and DE only under high-intensity, short-duration rainfall type. FR and F% were mainly affected by wind speed and the maximum 30-min rainfall intensity under low-intensity, long-duration rainfall type. At the intra-event scale, for both tree species, the mean lag time between the start of rainfall and stemflow was the shortest under high-intensity, short-duration rainfall type, while the mean duration and amount of stemflow after rain cessation were the greatest under high-amount, long-duration rainfall type. The relationship between stemflow intensity and rainfall intensity at the 5-min interval scale also depended greatly on rainfall type. These findings can help clarify stemflow dynamics and driving factors at both inter- and intra-event scales, and also provide abundant data and parameters for ecohydrological simulations in subtropical forests.  相似文献   
5.
In 1994, a network of small catchments (GEOMON) was established in the Czech Republic to determine input–output element fluxes in semi-natural forest ecosystems recovering from anthropogenic acidification. The network consists from 16 catchments and the primary observations of elements fluxes were complemented by monitoring of biomass stock, element pools in soil and vegetation, and the main water balance components. Over last three decades, reductions of SO2, NOx and NH3 emissions were followed by sulphur (S) and nitrogen (N) deposition reductions of 75% and 30%, respectively. Steeper declines of strong acid anion concentrations compared to cations (Ca, Mg, Na, K, NH4) in precipitation resulted in precipitation pH increase from 4.5 to 5.2 in bulk precipitation and from 4.0 to 5.1 in spruce throughfall. Stream chemistry responded to changes in deposition: S leaching declined. However at majority of catchments soils acted as a net source of S to runoff, delaying recovery. Stream pH increased at acidic streams (pH < 6) and aluminium concentration decreased. Stream nitrate (NO3) concentration declined by 60%, considerably more than N deposition. Stream NO3 concentration was tightly positively related to stream total dissolved nitrogen to total phosphorus (P) ratio, suggesting the role of P availability on N retention. Trends in dissolved organic carbon fluxes responded to both acidification recovery and to runoff temporal variation. An exceptional drought occurred between 2014 and 2019. Over this recent period, streamflow decreased by ≈ 40% on average compared to 1990s, due to the increases of soil evaporation and vegetation transpiration by ≈ 30% and declines in precipitation by ≈ 15% on average across the elevational gradient. Sharp decreases of stream runoff at catchments <650 m a.s.l. corresponded to areas of recent forest decline caused by bark beetle infestation on drought stressed spruce forests. Understanding of the interactions among legacies of acidification and eutrophication, drought effects on the water cycle and forest disturbance dynamics is requisite for effective management of forested ecosystems under anthropogenic influence.  相似文献   
6.
超大陆演化是地质研究的重要内容,华北克拉通与不同地质历史时期超大陆汇聚与裂解的联系对反演华北克拉通构造演化历史具有重要意义。本文在辽吉古元古代造山带中段的原划分为辽河群地层中首次识别出一套早古生代沉积建造。这套沉积建造与华北克拉通以浅海相的碳酸盐岩为主的早古生代沉积并不一致,以发育大量的陆源碎屑沉积为特征。我们对2件细砂岩分别进行了锆石LA-ICP-MS和SHRIMP U-Pb定年。定年结果显示,2件样品的最小年龄分别为~482Ma和~498Ma,反映了它们的最大沉积时代。2件样品的碎屑锆石年龄主要介于1600~500Ma,缺乏亲华北的物源信息,表明它们的物源主要来自于华北之外。2件样品年龄谱中最重要的峰值出现在格林威尔期和泛非期,表明华北克拉通曾与罗迪尼亚超大陆和冈瓦纳大陆存在联系。格林威尔期碎屑锆石可能来自于罗迪尼亚超大陆时期波罗地古陆物质在华北克拉通东缘的再循环;泛非期碎屑锆石可能来自于东冈瓦纳大陆的北缘造山带。  相似文献   
7.
Atmospheric dust is an integral component of the Earth system with major implications for the climate, biosphere and public health. In this context, identifying and quantifying the provenance and the processes generating the various types of dust found in the atmosphere is paramount. Isotopic signatures of Pb, Nd, Sr, Zn, Cu and Fe are commonly used as sensitive geochemical tracers. However, their combined use is limited by the lack of (a) a dedicated chromatographic protocol to separate the six elements of interest for low‐mass samples and (b) specific reference materials for dust. Indeed, our work shows that USGS rock reference materials BHVO‐2, AGV‐2 and G‐2 are not applicable as substitute reference materials for dust. We characterised the isotopic signatures of these six elements in dust reference materials ATD and BCR‐723, representatives of natural and urban environments, respectively. To achieve this, we developed a specific procedure for dust, applicable in the 4–25 mg mass range, to separate the six elements using a multi‐column ion‐exchange chromatographic method and MC‐ICP‐MS measurements.  相似文献   
8.
利用最新发布的CALIPSO产品,构建了2007-2017年中国沙尘气溶胶的三维分布,并结合HYSPLIT-4模式和再分析数据,探讨了沙尘的三维输送过程。结果表明:中国的沙尘排放源区主要是塔克拉玛干沙漠和巴丹吉林沙漠,沙尘气溶胶出现频率分别为60%和35%。塔克拉玛干沙漠排放的沙尘主要(50%~70%)停留在源地0~6 000 m高度,少部分向东输送至甘肃和内蒙古;巴丹吉林沙漠排放的沙尘则主要向东输送。中国沙尘排放量在春季最大,向东输送最强;夏季,东亚夏季风限制了沙尘向东输送;秋季,沙尘排放减弱,输送强度和夏季相当;沙尘排放量在冬季最小,输送最弱。夏季,沙尘在输送过程中可被抬升至高度5 000 m以上,春季次之,秋、冬季的沙尘主要在低层大气输送。沙尘在向东输送的过程中被抬升并和当地人为污染物混合变为污染性沙尘,华北地区污染性沙尘出现频率高达30%;输送到海洋的沙尘也会与洋面上(0~3 000 m高度)的海盐气溶胶混合,出现频率约为10%。  相似文献   
9.
基于地缘政治视角,分析本世纪初发生在原苏联地区“颜色革命”的诱发因素,认为美国根据其地缘战略格局对“颜色革命”发生地存在一定程度的主观选择性,国家内部经济、政治、社会等层面的矛盾也同样作为发生背景。在中亚地缘格局动态分析的基础上,结合中亚五国形势,从时间和空间双重维度对中亚地区未来发生“颜色革命”的可能性进行识别与评判,得出1) 整体来看,中亚近期内爆发“颜色革命”可能性较小,但从长远来看不能掉以轻心。2)土、乌未来稳定可期,塔、吉、哈需谨防“颜色革命”卷土重来。  相似文献   
10.
首先利用ALOS PALSAR数据,通过D-InSAR技术获取2007-06-03云南宁洱MS6.4地震的同震形变场,然后基于Okada弹性半空间位错模型反演该地震的断层几何以及精细滑动分布,最后计算宁洱地震后周边断层的静态库仑应力变化。结果表明,形变主要集中在西盘,最大视线向形变量为51.6 cm;反演得到的震源位置为23.05°N、101.02°E,深度3 km,断层走向145°,倾向49.5°,平均滑动角153°,发震断层为NNW向普洱断裂,断层活动以右旋走滑为主,兼具逆冲分量;断层面最大滑动量为1.2 m,反演得到的震级为MW619。基于库仑应力场发现,磨黑断裂处于库仑应力增加区域,而2014年景谷地震位于负值区域。结合实地考察资料和反演结果表明,宁洱地震为浅源地震,但断层并未出露地表。  相似文献   
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