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1.
Nina Kirchner Riko Noormets Jakob Kuttenkeuler Elias Strandell Erstorp Erik Schytt Holmlund Gunhild Rosqvist Per Holmlund Marika Wennbom Torbjrn Karlin 《第四纪科学杂志》2019,34(6):452-462
In Arctic alpine regions, glacio‐lacustrine environments respond sensitively to variations in climate conditions, impacting, for example,glacier extent and rendering former ice‐contact lakes into ice distal lakes and vice versa. Lakefloors may hold morphological records of past glacier extent, but remoteness and long periods of ice cover on such lakes make acquisition of high‐resolution bathymetric datasets challenging. Lake Tarfala and Kebnepakte Glacier, located in the Kebnekaise mountains, northern Sweden, comprise a small, dynamic glacio‐lacustrine system holding a climate archive that is not well studied. Using an autonomous surface vessel, a high‐resolution bathymetric dataset for Lake Tarfala was acquired in 2016, from which previously undiscovered end moraines and a potential grounding line feature were identified. For Kebnepakte Glacier, structure‐from‐motion photogrammetry was used to reconstruct its shape from photographs taken in 1910 and 1945. Combining these methods connects the glacial landform record identified at the lakefloor with the centennial‐scale dynamic behaviour of Kebnepakte Glacier. During its maximum 20th century extent, attained c. 1910, Kebnepakte Glacier reached far into Lake Tarfala, but had retreated onto land by 1945, at an average of 7.9 m year–1. Copyright © 2019 John Wiley & Sons, Ltd. 相似文献
2.
Changes in Arctic clouds during intervals of rapid sea ice loss 总被引：2，自引：0，他引：2
We investigate the behavior of clouds during rapid sea ice loss events (RILEs) in the Arctic, as simulated by multiple ensemble projections of the 21st century in the Community Climate System Model (CCSM3). Trends in cloud properties and sea ice coverage during RILEs are compared with their secular trends between 2000 and 2049 during summer, autumn, and winter. The results suggest that clouds promote abrupt Arctic climate change during RILEs through increased (decreased) cloudiness in autumn (summer) relative to the changes over the first half of the 21st century. The trends in cloud characteristics (cloud amount, water content, and radiative forcing) during RILEs are most strongly and consistently an amplifying effect during autumn, the season in which RILEs account for the majority of the secular trends. The total cloud trends in every season are primarily due to low clouds, which show a more robust response than middle and high clouds across RILEs. Lead-lag correlations of monthly sea ice concentration and cloud cover during autumn reveal that the relationship between less ice and more clouds is enhanced during RILEs, but there is no evidence that either variable is leading the other. Given that Arctic cloud projections in CCSM3 are similar to those from other state-of-the-art GCMs and that observations show increased autumn cloudiness associated with the extreme 2007 and 2008 sea ice minima, this study suggests that the rapidly declining Arctic sea ice will be accentuated by changes in polar clouds. 相似文献
3.
Marika Marnela Bert Rudels K. Anders Olsson Leif G. Anderson Daniel J. Torres James H. Swift 《Progress in Oceanography》2008,78(1):1-11
To determine the exchanges between the Nordic Seas and the Arctic Ocean through Fram Strait is one of the most important aspects, and one of the major challenges, in describing the circulation in the Arctic Mediterranean Sea. Especially the northward transport of Arctic Intermediate Water (AIW) from the Nordic Seas into the Arctic Ocean is little known. In the two-ship study of the circulation in the Nordic Seas, Arctic Ocean - 2002, the Swedish icebreaker Oden operated in the ice-covered areas in and north of Fram Strait and in the western margins of Greenland and Iceland seas, while RV Knorr of Woods Hole worked in the ice free part of the Nordic Seas. Here two hydrographic sections obtained by Oden, augmented by tracer and velocity measurements with Lowered Acoustic Doppler Current Profiler (LADCP), are examined. The first section, reaching from the Svalbard shelf across the Yermak Plateau, covers the region north of Svalbard where inflow to the Arctic Ocean takes place. The second, western, section spans the outflow area extending from west of the Yermak Plateau onto the Greenland shelf. Geostrophic and LADCP derived velocities are both used to estimate the exchanges of water masses between the Nordic Seas and the Arctic Ocean. The geostrophic computations indicate a total flow of 3.6 Sv entering the Arctic on the eastern section. The southward flow on the western section is found to be 5.1 Sv. The total inflow to the Arctic Ocean obtained using the LADCP derived velocities is much larger, 13.6 Sv, and the southward transport on the western section is 13.7 Sv, equal to the northward transport north of Svalbard. Sulphur hexafluoride (SF6) originating from a tracer release experiment in the Greenland Sea in 1996 has become a marker for the circulation of AIW. From the geostrophic velocities we obtain 0.5 Sv and from the LADCP derived velocities 2.8 Sv of AIW flowing into the Arctic. The annual transport of SF6 into the Arctic Ocean derived from geostrophy is 5 kg/year, which is of the same magnitude as the observed total annual transport into the North Atlantic, while the LADCP measurements (19 kg/year) imply that it is substantially larger. Little SF6 was found on the western section, confirming the dominance of the Arctic Ocean water masses and indicating that the major recirculation in Fram Strait takes place farther to the south. 相似文献
4.
Francois Gelin Marika D. Kok Jan W. de Leeuw Jaap S. Sinninghe Damst 《Organic Geochemistry》1998,29(8):1837-1848
To understand more fully the mode of preservation of organic matter in marine sediments, laboratory sulfurisation of intact cells of the cultured microalga Nannochloropsis salina was performed using inorganic polysulfides in seawater at 50°C. Solvent extractable and non-extractable materials were analysed by GC–MS and Py–GC–MS, respectively, to study the incorporation of sulfur into the microalgal organic matter. No GC-amenable sulfur-containing compounds were found in the extracts apart from some minor thiophenes with a phytanyl carbon skeleton. The residue after extraction and hydrolysis contained abundant macromolecular sulfur-containing moieties as revealed by the presence of dominant C28–C32 thiols, thiophenes, thianes and thiolanes in the flash pyrolysates. These products are thought to be formed from moieties derived from sulfurisation of C28–C32 diols and alkenols, characteristic lipids of N. salina. C1–C2 alkylated thiophenes were also found in the pyrolysates and probably result from moieties formed upon sulfurisation of carbohydrates. The highly resistant biomacromolecule (algaenan) synthesised by N. salina remains unaffected by sulfurisation. The non-hydrolysable residue isolated from the sulfurised N. salina thus comprises algaenan and (poly)sulfide-bound long alkyl chains. The sulfurisation experiments show that both selective preservation of algaenans and lipid and carbohydrate “vulcanisation” can be involved in the preservation of algal organic matter in marine environments. 相似文献
5.
Arctic sea ice mass budgets for the twentieth century and projected changes through the twenty-first century are assessed from 14 coupled global climate models. Large inter-model scatter in contemporary mass budgets is strongly related to variations in absorbed solar radiation, due in large part to differences in the surface albedo simulation. Over the twenty-first century, all models simulate a decrease in ice volume resulting from increased annual net melt (melt minus growth), partially compensated by reduced transport to lower latitudes. Despite this general agreement, the models vary considerably regarding the magnitude of ice volume loss and the relative roles of changing melt and growth in driving it. Projected changes in sea ice mass budgets depend in part on the initial (mid twentieth century) ice conditions; models with thicker initial ice generally exhibit larger volume losses. Pointing to the importance of evolving surface albedo and cloud properties, inter-model scatter in changing net ice melt is significantly related to changes in downwelling longwave and absorbed shortwave radiation. These factors, along with the simulated mean and spatial distribution of ice thickness, contribute to a large inter-model scatter in the projected onset of seasonally ice-free conditions. 相似文献
6.
Marika Haupt Michael Friedrich Vladimir V. Shishov Tatjana Boettger 《Climatic change》2014,122(1-2):201-215
Tree-ring oxygen stable isotope data series from conifers growing on the Dachstein Plateau (Austrian Alps) were selected to demonstrate the applicability of the serial pooling method using shifted 5-year tree-ring blocks for summer temperature reconstruction. The addressed method allows the construction of long isotope chronologies with significant climate correlation and well preserved climate sensitivity applying the irreducible sample replication of five trees. The linear regression model for temperature reconstruction is verifiable and the predicted data are well correlated with instrumental data, especially reproducing the long-term temperature trend. However, the reduced mean variance leads to loss of extreme years, which can be regulated by the combination of one data series in annual resolution with five shifted 5-year block data series. This significantly improves the variance of the mean chronology, sufficiently to identify extremes. Therefore, we recommend the use of mixed data sets as a compromise between essential sample replication and economic considerations. 相似文献
7.
The Arctic’s rapidly shrinking sea ice cover: a research synthesis 总被引：21，自引：1，他引：20
Julienne C. Stroeve Mark C. Serreze Marika M. Holland Jennifer E. Kay James Malanik Andrew P. Barrett 《Climatic change》2012,110(3-4):1005-1027
The sequence of extreme September sea ice extent minima over the past decade suggests acceleration in the response of the Arctic sea ice cover to external forcing, hastening the ongoing transition towards a seasonally open Arctic Ocean. This reflects several mutually supporting processes. Because of the extensive open water in recent Septembers, ice cover in the following spring is increasingly dominated by thin, first-year ice (ice formed during the previous autumn and winter) that is vulnerable to melting out in summer. Thinner ice in spring in turn fosters a stronger summer ice-albedo feedback through earlier formation of open water areas. A thin ice cover is also more vulnerable to strong summer retreat under anomalous atmospheric forcing. Finally, general warming of the Arctic has reduced the likelihood of cold years that could bring about temporary recovery of the ice cover. Events leading to the September ice extent minima of recent years exemplify these processes. 相似文献
8.
Microscopic distribution and speciation of Na, Mg, Ni and Cs in a simulated (inactive) nuclear waste glass were studied using micro X-ray fluorescence (μ-XRF) and micro X-ray absorption spectroscopy (μ-XAS), after aqueous leaching during 12 years at 90 °C. Na and Mg are major constituents of the glass that can be used to determine the progress of the glass corrosion process and the nature of secondary alteration phases. Ni and Cs represent dose determining long-lived radionuclides (59Ni, 135Cs) in vitrified nuclear waste.The Na-Mg μ-XRF maps revealed that the core regions of the glass fragments are apparently unaltered and compositionally homogeneous, whereas rims and interstitial spaces are enriched with Mg-rich smectite formed during the leaching process. The micro X-ray absorption near edge structure (μ-XANES) spectra collected at the Mg K-edge in the altered zones show three sharp resonances typical for crystalline Mg-silicates. These resonances are distinctive of Mg occupying undistorted octahedral positions. In contrast, the μ-XANES spectra collected in the core zones of the glass fragments lack this resonance pattern and are identical to the spectra measured on the pristine (unleached) MW glass.Micro extended X-ray absorption fine structure (μ-EXAFS) and μ-XANES analyses at the Ni K-edge revealed three distinct Ni(II) species: (a) Ni uniformly distributed in the glass matrix, (b) micro-inclusions with high Ni concentrations and (c) Ni associated to the Mg-clay. The comparison with reference spectra of unleached MW and other Ni-bearing silicate glasses indicated that species (a) represents the original coordinative environment of Ni in the glass. The μ-EXAFS analyses revealed that species (b) is structural Ni in trevorite (NiFe2O4), which probably formed through unmixing processes during the cooling of the glass melt. The μ-EXAFS of species (c) could be successfully modeled assuming specific adsorption or incorporation of Ni into the lattice of trioctahedral Mg-clay minerals. Alternative models assuming other elements (Ni, Al, Fe) in addition to Mg in the second shell could not be fitted successfully.Aqueous concentration data were used to calculate the speciation of the leaching solutions. Saturation index (SI) calculations indicate undersaturation with respect to NiCO3 and NiSO4·7H2O, but oversaturation with respect to β-Ni(OH)2. The latter result is probably due to the omission of Ni borate and Ni silicate complexes in the speciation calculations, for which formation constants are not available. With the help of estimation techniques, we could infer that such complexes would dominate the Ni speciation and consequently reduce the SI below the saturation of β-Ni(OH)2.The μ-XRF maps show that Cs is uniformly distributed in the MW glass, since no region with high Cs concentration could be detected. The Cs LIII-edge μ-XAS spectra were all very similar independently of the degree of alteration, indicating similar coordination environments of Cs in the core regions of the glass as well as in the secondary clays. These spectra largely differ from that measured for pollucite (a potential secondary Cs-phase in altered glasses) implying that the coordination environments of Cs in the MW glass and in pollucite are fundamentally different.The present study shows that μ-XRF and μ-XAS are essential tools in determining the fate and the retention mechanisms of radionuclides released from nuclear waste during aqueous alteration. Our spectroscopic analyses allowed us to exclude formation of specific Ni and Cs secondary solids (e.g. nepouite, β-Ni(OH)2, pollucite) during the aqueous alteration. Ni and Cs are instead distributed as trace elements in the alteration phases formed by major elements during the leaching process. Our results imply that solid solution and/or adsorption equilibria, rather than pure phase solubility equilibria, are the adequate chemical models to determine Ni and Cs aqueous concentrations in performance assessments for radioactive waste repositories. 相似文献
9.
Marika P. Dalton I. Matthew Watson Patricia A. Nadeau Cynthia Werner William Morrow Jeremy M. Shannon 《Journal of Volcanology and Geothermal Research》2009
Digital cameras, sensitive to specific regions of the ultra-violet (UV) spectrum, have been employed for quantifying sulfur dioxide (SO2) emissions in recent years. The instruments make use of the selective absorption of UV light by SO2 molecules to determine pathlength concentration. Many monitoring advantages are gained by using this technique, but the accuracy and limitations have not been thoroughly investigated. The effect of some user-controlled parameters, including image exposure duration, the diameter of the lens aperture, the frequency of calibration cell imaging, and the use of the single or paired bandpass filters, have not yet been addressed. In order to clarify methodological consequences and quantify accuracy, laboratory and field experiments were conducted. Images were collected of calibration cells under varying observational conditions, and our conclusions provide guidance for enhanced image collection. Results indicate that the calibration cell response is reliably linear below 1500 ppm m, but that the response is significantly affected by changing light conditions. Exposure durations that produced maximum image digital numbers above 32 500 counts can reduce noise in plume images. Sulfur dioxide retrieval results from a coal-fired power plant plume were compared to direct sampling measurements and the results indicate that the accuracy of the UV camera retrieval method is within the range of current spectrometric methods. 相似文献
10.
Contaminant exposure and effects in Baltic ringed and grey seals as assessed by biomarkers 总被引：3，自引：0，他引：3
Nyman M Bergknut M Fant ML Raunio H Jestoi M Bengs C Murk A Koistinen J Bäckman C Pelkonen O Tysklind M Hirvi T Helle E 《Marine environmental research》2003,55(1):73-99
The Baltic Sea ecosystem has suffered from a heavy pollutant load for more than three decades. Persistent organic pollutants (POPs) and heavy metals have been of most concern due to their persistence and toxic properties. Ringed seals (Phoca hispida baltica) and grey seals (Halichoerus grypus) living in the Baltic Sea have been suffering from pathological impairments, including reproductive disturbances, which have resulted in a depressed reproductive capacity. We investigated several biochemical parameters as potential biomarkers for exposure to and effects of the contaminant load in the Baltic seals. Seals from less polluted areas were used as reference material in terms of the pollution load. In both Baltic seal populations, the levels of some biochemical parameters diverged from those in the reference seals, and some of these showed a clear correlation with the individual contaminant load. Of the potential bioindicators, we propose cytochrome P4501A activity and vitamin E levels, in blubber or plasma, as exposure biomarkers for polychlorinated biphenyls (PCBs) and dichlorodiphenyltrichloroethane (DDT) in both species. The arylhydrocarbon receptor-mediated chemical-activated luciferase gene expression (CALUX) response reflects the whole PCB and DDT burden in ringed seals. Retinyl palmitate (vitamin A) levels showed a negative correlation with the individual POP load, and is proposed as potential effect biomarkers for the depletion of the vitamin A stores. As the nutritional levels of both vitamin A and E have an impact on the vitamin levels in the seals, more information on the dietary vitamin levels is needed before any conclusions can be drawn. As the relationship between biochemical parameters and contaminants varied between the two species, species-specific characteristics has to be considered when monitoring the health status and possible toxic effects of the contaminant load in ringed and grey seals. 相似文献