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1.
北极黄河站秋季气团传输影响下大气气溶胶数谱分布特征   总被引:2,自引:2,他引:0  
2013 年9月在北极黄河站开展了气溶胶数谱(10~400nm)的短期观测实验。数浓度小时平均值主要出现在300~400cm-3,平均值为350cm-3,高于新奥尔松Zeppelin 全球大气本底站及环北极海洋大气7-9月航测报道的浓度。大气气溶胶的三个模态(核模态、爱根核模态和积聚模态)数浓度平均分别为35、122和193cm-3。观测期间没有发生新粒子生成事件,平均数谱分布呈现双模态的分布特征,模态峰值分别出现在30nm和115nm,由积聚模态主导。平均数谱分布的几何中值粒径出现在约100~110nm。从单颗粒分析结果来看,观测期间黄河站地区大气气溶胶主要以海盐气溶胶为主,但是在来自挪威海域和北欧大陆的气团影响下,也观测到煤烟颗粒、富硫颗粒物和含碳颗粒物等人为气溶胶。  相似文献   

2.
利用飞机航测于2018年夏季在东北吉林省用宽范围粒径谱仪对10 nm~10μm大气颗粒物的数浓度谱进行在线监测,分析大气颗粒物的垂直分布廓线和粒径分布特征。结果表明,东北地区近地面颗粒物数浓度为5.8×10~3~9.9×10~(4)cm~(-3),平均值为(2.7±2.2)×10~(4)cm~(-3);垂直方向上颗粒物数浓度随海拔升高整体呈降低趋势,且垂直廓线存在两种类型:一种是在边界层附近存在较明显的分界线,即在边界层下方,大气颗粒物数浓度随高度升高而显著降低,在边界层上方,大气颗粒物数浓度变化随高度变化不明显;第二种是随高度的升高,城市上空的大气颗粒物数浓度降低,且海拔高度与大气颗粒物数浓度呈现近似线性负相关的关系。在观测期间,颗粒物的粒径大多集中在爱根模态,其峰值位于25~30 nm,后向气流轨迹显示,气团来源于蒙古及内蒙古地区。在四平城市上空观测到1例新粒子生成事件,其核模态颗粒物数浓度为当日其他地区的4倍,后向气流轨迹显示其气团来源于中国辽宁省且受局地气团影响。  相似文献   

3.
210Pb等核素对于大气物质传输途径、流域侵蚀作用和水体沉积过程有重要示踪价值.认识它们在环境运移过程的作用机理、速率和通量是示踪研究的基本内容.我们最新的研究进展主要有1)取得采样及分析数据的国际可比性;2)揭示黔中地区近地面空气210Pb呈现高浓度U型年分布特征;3)获得青海瓦里及山关顶部7Be的高浓度分布;气流强下沉影响在观风山的滞后性和低海拔气团上升影响在瓦里关山的滞后性;4)模拟显示210Pb在一些地区近地面空气的高浓度分布和在全球的高沉降通量环带分布;5)揭示富营养湖泊出现的微粒清洗效应及210Pbex对湖泊生产力变化的示踪价值.  相似文献   

4.
瓦里关山与观风山近地面空气7Be浓度季节性变化对比   总被引:4,自引:0,他引:4  
7Be广泛应用于大气物质传输、表土季节性迁移和微粒混合作用的示踪。它在不同地域空气中的浓度分布构成了多领域研究的基础。7Be在对流层空气中的浓度随地表海拔高度而增加。基于瓦里关山和观风山的位置差异和海拔高差,对比观测其近地面空气7Be浓度变化不仅有益于区域尺度的大气和地表环境过程的示踪,而且对全球尺度的研究也将具重要意义。2002-10-09~2004-01-21,利用美国环境测量实验室的低水平核素表层大气采样系统在瓦里关山和观风山同步连续进行每周1个大气气溶胶样品的采集工作。7Be的比活度系用多道能谱仪进行γ谱测定,测量误差小于6%。中美两实验室对逐周样品测量结果表明两实验室的数据具有很好的可比性。两个站点7Be浓度逐周变化趋势总体相似,具有2~6周的短周期波动,波峰与波谷具有良好的对应关系,其高值或低值波动延迟或超前的差异与区域尺度的天气过程传播一致。瓦里关山和观风山7Be的年均浓度分别为(14.7±1.5)mBq/m3和(4.1±0.9)mBq/m3,前者约为后者的3.6倍。近地面空气7Be浓度与同期降水量的比较表明,在周时间尺度上,两者呈现出较好的预期负相关变化;而在月平均尺度上,两地7Be浓度变化比较稳定。位于内陆地区的瓦里关山受低海拔气团上升的影响较小,其空气中7Be浓度变化较真实地反映了中纬度、高海拔地区的背景水平。观风山地区虽然受到低纬度海洋性上升气团的影响,但7Be浓度变化仍然显示出低纬度、较高海拔地区的预期水平。  相似文献   

5.
北京市大气颗粒物中全氟烷基化合物的粒径分布特征   总被引:2,自引:1,他引:1  
人为排放的持久性有机污染物倾向于在细级大气颗粒物中富集,但目前国内外关于大气颗粒物中全氟烷基化合物(PFASs)粒径分布在不同国家地区有显著差异,而在我国北京地区PFASs在不同粒径大气颗粒物中的富集能力尚不清楚。本文采用五级大流量主动分级采样器采集了北京市大气颗粒物样品,利用超声萃取结合高效液相色谱-电喷雾负电离源串联质谱测定PFASs含量,探讨了该地区大气颗粒物中PFASs的浓度水平和粒径分布特征,以及大气颗粒物浓度变化对PFASs浓度变化的影响。结果表明:研究区∑PFASs范围为10. 1~62. 9 pg/m3,76. 4%~83. 8%的PFASs集中分布在PM2. 5颗粒物中,其中含量较高的PFOA、PFNA和PFDA在0. 25μm细颗粒物中占比最高,分别为26. 3%~43. 7%、30. 3%~68. 6%和30. 6%~49. 7%; PFOS在0. 25μm细颗粒物中没有检出,主要分布在1~2. 5μm和0. 25~1μm颗粒物中。此外,研究发现北京市霾天大气颗粒物中∑PFASs为晴天的3. 5倍,且不同粒径大气颗粒物浓度变化对PFASs各化合物表现出不同的富集能力,其中PFOA、PFOS、PFNA和PFDA等中链PFASs更易富集。  相似文献   

6.
认识环境核素在不同地域空气中的浓度分布和沉降到地表环境的通量对气溶胶污染物全球扩散模型的建立和验证、沉积过程示踪和沉积计年、流域侵蚀示踪参比,以及生态系统受天然辐照的评价等多个领域都是关键的依据.自2001年以来在贵阳观风山等地逐周连续采样,对近地面空气和降水中210Pb和7Be浓度的观测结果表明:①因气象条件变化,近地面空气210mPb和7Be周浓度具有2~6周变幅不等的短周期波动.210Pb空气浓度在年内的总趋势呈现出受气温变化的总体影响和降水的短暂调控;而7Be空气浓度出现连续不断的峰-谷交替.②两核素在近地面空气周浓度的低值同步,210Pb/7Be比率较高(≥0.8),显示出海洋性贫210Pb-7Be气团的入侵影响;它们高的周浓度也同步耦合,比率较低(≤0.7),显示出高层大气富7Be气团的输入.③210Pb和7Be的周降水浓度及水-气分配系数在秋末春季较高,而春末-秋季明显偏低.周降水浓度随同期空气浓度呈增高趋势,其季节分界分别为0.2 Bq/L和1 Bq/L;而Kd值随同期空气浓度增大呈降低趋势.210Pb和7Be的降水沉降主要分布在每年的春夏季;周沉降量随同期降水量呈增大趋势,7Be增大的斜率约为210Pb的3倍;当近于零降水时,它们在降水中的初始比率约为2.5.它们出现高或者较高的周降水沉降都伴随当周或邻周空气浓度的急剧下降;降水中210Pb/7Be比率主要分布在≤0.5,并与空气中210Pb/7Be比率基本同步,显示出两核素被降水清洗的效率基本相近.④2008年冰冻极端天气过程中,210Pb-7Be空气浓度同步低谷并存在气溶胶低浓度与高比活度耦合.⑤观风山7Be周空气浓度显示低纬度、较高海拔地区的预期水平;短周期波动反映强下沉气流和低海拔上升气团影响分别在观风山和瓦里关山的滞后性.  相似文献   

7.
自2001年12月连续逐周在贵阳观风山附近对近地面空气210Pb-7Be浓度和沉降量的观测表明:区域性降水和气温制约近地面空气210Pb具高浓度"U"型年分布;降水量和平流层向下输送影响近地面空气7Be月均浓度的季节性变化;210Pb/7Be月均浓度比率受控于210Pb变化和富7Be气团下沉的影响.观风山与瓦里关山之间因纬度和海拔的关系,7Be比率急剧震荡,显示出海洋性贫7Be气团入侵对观风山地区的明显影响.2002-2008年间贵阳观风山近地面空气210Pb的年均浓度(2.8±0.6)mBq/m3,约为全球若干站点中最高平均浓度值的4倍;而7Be的年均浓度(4.8±0.6)mBq/m3,与全球高海拔站点长期观测的平均值相当,大约为北半球中纬度对流层顶部附近7Be浓度值(18.0 mBq/m3)的1/3.8,显示出低纬度、较高海拔地区的预期水平.2003年,瓦里关山和观风山近地面空气7Be的年均浓度比为3.8,与预期的大气输送和混合作用基本一致.7Be月均浓度的增大趋势反映出受太阳黑子数减少的变化关系,其影响底线大约为4 mBq/m3;7Be年均浓度波动的增大趋势反映出受太阳黑子数降低的可能影响.贵阳观风山降水中7Be和210Pb的体积加权浓度分别为0.72 Bq/L和0.27 Bq/L;年沉降通量分别为0.080 Bq/(cm2·a)和0.031 Bq/(cm2·a).数值模拟显示出全球空气210Pb高浓度区和高沉降通量环带分布,印证了洱海和红枫湖沉积物7Be和157Cs蓄积的模拟结果.  相似文献   

8.
基于2017年1月4日至7日成都市一次重霾污染过程的系留汽艇探测的低层大气气象要素和大气颗粒物垂直探空加密观测资料,分析了大气边界层结构及气溶胶垂直分布。结果表明,此次重霾污染期间,大气边界层昼夜变化特征基本消失。稳定边界层结构出现25次,对流边界层结构仅出现3次,大气边界层结构趋于稳定,边界层高度普遍在700 m以下。霾污染发生、维持及消散阶段大气边界层气溶胶垂直结构具有明显差异。霾污染发生阶段,大气边界层气溶胶粗、细粒子主要集中在300m高度以下,近地面层大气气溶胶粒子累积触发霾污染事件;霾维持阶段,大气颗粒物粒子浓度数垂直方向趋于一致,大气边界层稳定结构中存在强的大气垂直混合作用;在霾消散阶段,较高处的气溶胶粒子浓度最先下降,且下降幅度最大,表明对流层自由大气作用对霾污染消散具有影响。大气边界层风速的增大加剧了大气传输扩散。温度与大气颗粒物浓度在近地层呈负相关关系,在100m高度以上呈正相关关系。大气边界层低层偏冷,高层偏暖的稳定大气热力层结减弱了大气污染物的垂直扩散。相对湿度的增加有利于气溶胶粒子的吸湿增长和液相化学反应,加剧了霾污染。  相似文献   

9.
张林  靳孟贵  刘延锋  梁杏  杨世琪  鲜阳 《地球科学》2021,46(8):2984-2998
研究典型区域大气温室气体的变化有助于有效应对气候变化、减缓全球变暖和减少极端气候事件.选取1997-2018年瓦里关和2009-2015年上甸子温室气体月值数据,应用线性趋势分析法和Mann-Kendall突变检验法分析两站温室气体的时间序列特征、季节变化趋势,构建HYSPLIT后向轨迹模型分析季风运输和大气边界层条件对温室气体的潜在影响.瓦里关和上甸子温室气体均逐年增长,具有明显的季节变化特征.两站CO2均在8月达到最低值,CH4则在8月达到峰值,SF6四季差异不大.瓦里关N2O在12月达到最高,6月降到最低;而上甸子N2O在7月达到峰值,9月降至最低.瓦里关和上甸子大气温室气体均受到局地生物源和非生物源、季风远距离运输、大气边界层条件和光化学过程等多种因素的共同作用.   相似文献   

10.
了解地震前后气体地球化学异常特征及其与地震和构造活动的关系,可为地震监测预报提供参考。本文在以瓦里关站数据验证AIRS反演产品可靠性的基础上,通过震中区不同高度CO体积混合比和异常指数法研究了2014年2月12日新疆于田Ms7.3地震前后CO的变化特征。结果表明,AIRS传感器和瓦里关站的CO观测结果具有一致的月、季、年时间变化特征,表明AIRS反演的CO数据可以真实可靠地反映近地表CO的变化特征。CO浓度在地震前及地震当月发生下降,地震次月CO浓度出现最大幅度的异常。CO浓度出现下降是地震孕育过程中断裂带弹性闭锁造成,地震引起地下排气增强和大气化学反应是CO浓度异常的原因。  相似文献   

11.
International unity is becoming ever stronger in this country owing to an increasing similarity in the development of the cultural environment. This comprises the provision of all the country's republics with a sufficient number of schools, theatres, and other institutions and cultural information media in accordance with the needs of the population. An important part is played by the rise in ‘the general educational level, as well as the level of professional qualifications and skills. Among all the Soviet nations and nationalities, this rise being more rapid among formerly backward peoples. Prominent among the factors of internationalization is the progressive development of the nationalities’ cultural resources, while professional culture is being increasingly brought within the reach of the masses.The implementation of the nationalities policy promotes the all-round development of all Soviet nations and nationalities, their drawing together, the upsurge of the individual capabilities of every Soviet citizen.  相似文献   

12.
It is known from observations that the center of mass of the Moon does not coincide with the geometric center of its figure, and the line connecting these two centers is not aligned with the direction toward the center of the Earth, instead deviating toward the Southeast. This stationary deviation of the axis of the inertia ellipsoid of the Moon to the South of the direction toward the Earth is analyzed. A system of five linear differential equations describing the physical libration of the Moon in latitude is considered, and these equations are derived using a new vector method taking into account perturbations from the Earth and partly from the Sun. The characteristic equation of this system is obtained, and all five oscillation frequencies are found. Special attention is paid to the fifth (zero) frequency, for which the solution of the latitude libration equations are stationary and represents a previously unknown additional motion of the rotational axis of theMoon in a cone with a small opening angle. In contrast to the astronomical precession of the Earth, the rotation of the angular-velocity vector is in the positive direction (counter-clockwise), with the period T 3 = 27.32 days. On this basis, this phenomenon has been named “quasi-precession.” This quasi-precession leads to a stationary inclination of the major axis of the inertia ellipsoid of theMoon to the South (for an observer on Earth), making it possible to explain one component of the observed deviation of the center of mass of the Moon from the direction toward the Earth. The opening angle of the quasiprecession cone is approximately 0.834″.  相似文献   

13.
14.
Chronological analyses of correlations between certain global repeating events (mass extinctions of marine organisms, meteorite impacts, and flashes in the frequency of geomagnetic reversals) during the Phanerozoic Eon and the motion of the solar system in the Galaxy are presented for five rotationally symmetrical models for the regular Galactic gravitational field. Thirteen of sixteen mass-extinction events can be described by a repetition interval of 183±3 million years. This is in agreement with the anomalistic period (interval between two subsequent passages of the Sun through the apocenter of its Galactic orbit) in the model of Allen and Martos. The positions of the minima and maxima in Gaussian functions approximating the frequency distribution for geomagnetic reversals also agree with the times of passage of the Sun through the apocenter and pericenter, respectively, of its Galactic orbit in this model. The maximum in the distribution of the deviations of the dates of mass extinctions from the nearest dates of impacts of large, crater-forming bodies is close to zero, providing evidence that many such events are correlated. As a rule, extinctions follow impact events. The impacts of large bodies have occurred most often when the solar system passes through the Galactic plane, while mass extinctions occur more often at some distance from the Galactic plane (about 40 pc). As a rule, intervals of increases in the frequency of geomagnetic reversals coincide with dates of impacts of large bodies. At the same time, these intervals do not show a clear correlation with the dates of mass extinctions. The intensity of mass extinctions, like the energy released by impacts, is consistently higher in periods when the Sun is moving from the apocenter toward the pericenter of its orbit, than when it is moving from the pericenter toward the apocenter. Thus, there is evidence for a variety of relationships between repeating global events in the Phanerozoic and the motion of the Sun in the Galaxy. Long-period variations in the frequency of geomagnetic reversals are correlated with the orbital motion of the Sun, and increases in the frequency of geomagnetic reversals are correlated with impacts. Mass extinctions are correlated with the impacts of large bodies, whose motions may have been perturbed by clouds of interstellar material concentrated toward the Galactic plane and by the shock front associated with the Perseus spiral arm, through which the solar system passes. The velocity of the Sun relative to the spiral pattern is estimated.  相似文献   

15.
从榴辉岩与围岩的关系论苏鲁榴辉岩的形成与折返   总被引:4,自引:1,他引:4       下载免费PDF全文
位于华北和扬子两板块碰撞带中的苏鲁榴辉岩形成的温压条件不但是超高压,而且是高温。榴辉岩的PTt轨迹表明其为陆-陆磁撞俯冲带的产物。榴辉岩的区域性围岩花岗质片麻岩为新元古代同碰撞期花岗岩,榴辉岩及其他直接围岩皆呈包体存在于其中,并见新元古代花岗岩呈脉状侵入榴辉岩包体中。区域性围岩新元古代花岗岩的锆石中发现有柯石英、绿辉石等包裹体,表明新元古代花岗岩的组成物质也经受过超高压变质作用,且榴辉岩与围岩新元古代花岗岩的锆石U-Pb体系同位素年龄基本相同。但新元古代花岗岩所记录的变质作用和变形作用期次(或阶段)却少于榴辉岩。椐上述可得如下推断:超高压榴辉岩与新元古代花岗岩岩浆是同时在碰撞带底部(俯冲板块前部)形成的;榴辉岩的第一折返阶段是由新元古代花岗岩岩浆携带上升的,其第二折返阶段是和新元古代花岗岩一起由逆冲及区域性隆起而上升,遭受剥蚀。  相似文献   

16.
某高速公路下伏煤矿采空区稳定性分析   总被引:10,自引:0,他引:10  
在论述某高速公路下伏砦脖煤矿采空区地质、采矿和工程地质特征的基础上, 进行了稳定性数值模拟分析, 定性与定量地分析与评价了该煤矿采空区的地表变形特征及稳定性。研究结果表明: 该煤矿采空区的变形尚未完成, 对拟建的高速公路将产生很大的危害, 必须采取相应的工程治理措施。   相似文献   

17.
18.
摩擦桩基桩土间极限摩阻力取值问题探讨   总被引:1,自引:0,他引:1  
陈银生 《世界地质》1999,18(1):54-59
通过对广珠东线高速公路横沥大桥的试桩及土体的工程地质条件分析,总结出影响摩擦桩基桩土间极限摩阻力取值的一般问题以及解决问题的方法和措施。  相似文献   

19.
In order to characterise the influence of the heavyrains on the observed landslides during the 1996–1997hydrological cycle, rainfall records for the last 100years are analysed from 104 stations in easternAndalusia. Regarding the amounts of rain recordedbetween October 1996 and March 1997 in the 104stations studied, 31 presented new all-time records;15 presented values that were 80–100% of thepre-1995 record; 49 stations, 80–50%; and 9stations, < 50%. A map has been devised of thesusceptibility of the materials through which thesouth-eastern Andalusian road network crosses,together with an inventory of the damage caused byinstability phenomena on banks and cuttings of theroad network during the winter of 1996–1997. Therelationships between the rainfall during the studyperiod, the damage caused to the road network and thesusceptibility of the materials affected are analysed.The results indicate that there is a clearcorrespondence between the rainfall recorded and thesusceptibility of the materials with the inventorieddamage. It is concluded that the widespread seriousdamage caused in early 1997 to the roads andsurrounding areas in the Alpujarra region and thecoast of the Province of Granada was mainly caused bythe extraordinarily heavy rains. However, considerablyless damage was observed where the susceptibility ofthe terrain is low, thus highlighting the extremeusefulness of terrain-susceptibility maps for riskprevention and territorial planning.  相似文献   

20.
The structure of the eastern Pyrenees consists mainly of south-directed thrusts involving basement and cover rocks. An antiformal stack developed by the piling up of basement thrust sheets which outcrop in the Axial zone. These structures account for a thin-skinned thrust model rather than a vertical fault model in which the Axial zone would be essentially autochthonous, and the North-Pyrenean fault the axial plane of a fan thrust system. New data from the Eastern Pyrenees and the thin-skinned model suggest that(1) the structure east of the Pedraforca nappe is similar to that of the Central Pyrenees; (2) the cover rocks of the South-Pyrenean units and of the Axial zone-after restoration—built up a northwards-thickening prism consistent with the existence of a unique Pyrenean sedimentary basin during Mesozoic time; (3) the Axial zone is only a complex antiformal stack developed as a part of South-Pyrenean system related to the Paleogene thrusting-tectonics. The Axial zone palaeogeographic area had no special meaning during Mesozoic time.  相似文献   

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