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1.
Xue  Tao  Liu  Jun  Zhang  Qiang  Geng  Guannan  Zheng  Yixuan  Tong  Dan  Liu  Zhu  Guan  Dabo  Bo  Yu  Zhu  Tong  He  Kebin  Hao  Jiming 《中国科学:地球科学(英文版)》2019,62(12):1847-1856
Exposure to fine particulate matter(PM_(2.5)) is known to harm public health.In China,after implementation of aggressive emissions control measures under the Action Plan of Air Pollution Prevention and Control(2013-2017),air quality has significantly improved.In this work,we investigated changes in PM_(2.5) exposure and the associated health impacts in China for the period 2013-2017.We used an optimal estimator of PM_(2.5) combining in-situ observations,satellite measurements,and simulations from a chemical transport model to derive the spatial and temporal variations in PM_(2.5) exposure,and then used welldeveloped exposure-response functions to estimate the premature deaths attributable to PM_(2.5) exposure.We found that national population-weighed annual mean PM_(2.5) concentrations decreased from 67.4μgm~(-3) in 2013 to 45.5μgm~(-3) in 2017(32%reduction).This rapid decrease in PM_(2.5) pollution led to a 14% reduction in premature deaths due to long-term exposure.We estimated that,during 2013-2017,the premature deaths attributable to long-term PM_(2.5) exposure decreased from 1.2 million(95% CI:1.0,1.3;fraction of total mortality:13%) in 2013 to 1.0 million(95% CI:0.9,1.2;10%) in 2017.Despite the rapid decrease in annual mean PM_(2.5) concentrations,health benefits associated with reduced long-term exposure were limited,because for many cities,the PM_(2.5) levels remain at the portion where the exposure-response function is less steeper than that at the lowconcentration end.We also found that the deaths associated with acute exposure decreased by 61% during 2013-2017 due to rapid reduction in the number of heavily polluted days.Our results confirm that clean air policies in China have mitigated the air pollution crisis;however,continuous emissions reduction efforts are required to protect citizens from air pollution.  相似文献   

2.
Wang  Yuesi  Li  Wenjie  Gao  Wenkang  Liu  Zirui  Tian  Shili  Shen  Rongrong  Ji  Dongsheng  Wang  Shuai  Wang  Lili  Tang  Guiqian  Song  Tao  Cheng  Mengtian  Wang  Gehui  Gong  Zhengyu  Hao  Jiming  Zhang  Yuanhang 《中国科学:地球科学(英文版)》2019,62(12):1857-1871
Accurate determination of the atmospheric particulate matter mass concentration and chemical composition is helpful in exploring the causes and sources of atmospheric enthalpy pollution and in evaluating the rationality of environmental air quality control strategies.Based on the sampling and chemical composition data of PM_(2.5) in different key regions of China in the CARE-China observation network,this research analyzes the environmental air quality data released by the China National Environmental Monitoring Centre during the studied period to determine the changes in the particulate matter mass concentration in key regions and the evolution of the corresponding chemical compositions during the implementation of the Action Plan for Prevention and Control of Air Pollution from 2013-2017.The results show the following.(1) The particulate matter mass concentration in China showed a significant downward trend;however,the PM_(2.5) annual mass concentration in 64% of cities exceeds the New Chinese Ambient Air Quality Standard(CAAQS) Grade Ⅱ(GB3095-2012).The region to the east of the Taihang Mountains,the Fenhe and Weihe River Plain and the Urumqi-Changji regions in Xinjiang,all have PM_(2.5) concentration loading that is still high,and heavy haze pollution occurred frequently in the autumn and winter.(2) During the heavy pollution in the autumn and winter,the concentrations of sulfate and organic components decreased significantly.The mean SO_4~(2-) concentration in PM_(2.5) decreased by 76%,12%,81% and 38% in Beijing-Tianjin-Hebei(BTH),the Pearl River Delta(PRD),the Sichuan-Chongqing region(SC) and the Fenhe and Weihe River Plain,respectively.The mean organic matter(OM) concentration decreased by 70%,44%,48% and 31%,respectively,and the mean concentration of NH_4~+ decreased by 68%,1.6%,38% and 25%,respectively.The mean elemental carbon(EC) concentration decreased by 84% and 20% in BTH and SC,respectively,and it increased by 61% and 11% in the PRD and Fenhe and Weihe River Plain,respectively.The mean concentration of mineral and unresolved chemical components(MI) dropped by 70%,24% and 13% in BTH,the PRD and the Fenhe and Weihe River Plain,respectively.The change in the PM_(2.5) chemical composition is consistent with the decrease of the PM_(2.5)mass concentration.(3) In 2015,the mean OM concentration contributions to fine particles and coarse particles were 13-46%and 46-57%,respectively,and the mean MI concentration contributions to fine particles and coarse and particles were 31-60%and 39-73%,respectively;these values are lower than the 2013 values from the key regions,which is the most important factor behind the decrease of the particulate matter mass concentration.From 2013 to 2015,among the chemical components of different particle size fractions,the peak value of the coarse particle size fraction decreased significantly,and the fine particle size fractions of SO_4~(2-),NO_3~-,and NH_4~+ decreased with the decrease of the particulate matter mass concentration in different particle size fractions.The fine-particle size peaks of SO_4~(2-),NO_3~-and NH_4~+ shifted from 0.65-1.1μm to the finer size range of0.43-0.65 μm during the same time frame.  相似文献   

3.
<正>China suffers from severe air pollution in the past decades,characterized by high-levels of fine particulate matter(PM_(2.5)) concentrations. To mitigate PM_(2.5) pollution, the Chinese government issued the Air Pollution Prevention and Control Action Plan (referred to as the Clean Air Action hereinafter) in 2013, which requires the three key regions,  相似文献   

4.
Gao  Ying  Wang  Lifang  Guo  Xianghui  Xu  Yi  Luo  Li 《中国科学:地球科学(英文版)》2020,63(9):1339-1352
At the global scale,atmospheric inputs of nitrogen are an important source of the new nitrogen that supports new marine production,especially in oligotrophic open oceans and marginal seas.This study reports quantities of atmospheric deposition of dissolved inorganic nitrogen(DIN) to the largest marginal sea in the North Pacific(the oligotrophic South China Sea,SCS) based primarily on rainwater sampling in the open northwestern region(Yongxing Island) from 2013 to 2015,and aerosol sampling from the SCS basin in June 2017.Atmospheric wet and dry deposition of DIN and their potential contributions to productivity were estimated.The volume-weighted mean rainwater concentrations during the wet and dry seasons were 4.9 and 18.1 μmol L~(-1) for N+N(NO_3~-+NO_2~-),and 5.7 and 4.0μmol L~(-1) for NH_4~+,respectively.Rainwater concentrations of DIN were lower in the marginal seas than in the open ocean.The aerosol NO_3~-concentration was 1.15±1.18 μg m~(-3) during the wet season,which is slightly lower than reported for the East China Sea and East Sea,but higher than in the Arabian Sea.Monthly wet and dry deposition rates ranged from 0.4-3.9 and 0.4-1.2 mmol m~(-2) mon~(-1) for NO_3~-,and 0.2-1.3 and 0.01-0.02 mmol m~(-2) mon~(-1) for NH_4~+,respectively.The annual wet and dry deposition fluxes of DIN were estimated to be 16.8 and 10.1 mmol m~(-2)yr~(-1),respectively.Compared to other marginal seas,the SCS receives less atmospheric NO_3~-inputs than the Yellow Sea,East China Sea,East Sea,and northeastern Mediterranean Sea.The total atmospheric DIN deposition may account for 1.8-11.1% of the nitrogen supporting new production and 0.7-1.8% of the nitrogen supporting primary production.  相似文献   

5.
A three-dimensional variational(3DVAR) data assimilation(DA) system is presented here based on a size-resolved sectional aerosol model, the Model for Simulating Aerosol Interactions and Chemistry(MOSAIC) within the Weather Research and Forecasting model coupled to Chemistry(WRF-Chem) model. The use of this approach means that both gaseous pollutants such as SO_2, NO_2, CO, and O_3 as well as particulate matter(PM_(2.5), PM_(10)) observational data can be assimilated simultaneously.Two one-month parallel simulation experiments were conducted, one with the assimilation of surface hourly concentration observations of the above six pollutants released by the China National Environmental Monitoring Centre(CNEMC) and one without assimilation in order to verify the impact of assimilation on initial chemical fields and subsequent forecasts. Results show that, in the first place, use of the DA system can provide a more accurate model initial field. The root-mean-square error of PM_(2.5), PM_(10), SO_2, NO_2, CO, and O_3 mass concentrations in analysis field fell by 29.27 μg m~(-3)(53.5%), 34.5 μg m~(-3)(50.9%),30.36 μg m~(-3)(64.2%), 8.91 μg m~(-3)(39.5%), 0.46 mg m~(-3)(47.4%), and 15.11 μg m~(-3)(51.0%), respectively, compared to a background field without assimilation. At the same time, mean fraction error was reduced by 42.6%, 53.1%, 45.2%, 43.1%,69.9%, and 48.8%, respectively, while the correlation coefficient increased by 0.51, 0.55, 0.48, 0.38, 0.47, 0.65, respectively.Secondly, the results of this analysis reveal variable benefits from assimilation on different pollutants. DA significantly improves PM_(2.5), PM_(10), and CO forecasts leading to positive effects that last more than 48 h. The positive effects of DA on SO_2 and O_3 forecasts last up to 8 h but that remains relatively poor for NO_2 forecasts. Thirdly, the influence of assimilation varies in different areas. It is possible that the positive effects of DA on PM_(2.5) and PM_(10) forecasts can last more than 48 h across most regions of China. Indeed, DA significantly improves SO_2 forecasts within 48 h over north China, and much longer CO assimilation benefits(48 h) are found in most regions apart from north and east China and across the Sichuan Basin. DA is able to improve O_3 forecasts within 48 h across China with the exception of southwest and northwest regions and the O_3 DA benefits in southern China are more evident, while from a spatial distribution perspective, NO_2 DA benefits remain relatively poor.  相似文献   

6.
Particle hygroscopicity plays a key role in understanding the mechanisms of haze formation and particle optical properties. The present study developed a method for predicting the effective hygroscopic parameter k and the water content of PM_(2.5) on the basis of the k-K?hler theory and bulk chemical components of PM_(2.5). Our study demonstrated that the effective hygroscopic parameter can be estimated using the PM_(2.5) mass concentration, water-soluble ions, and total water-soluble carbon. By combining the estimated k and ambient relative humidity, the water content of PM_(2.5) can be further estimated. As an example, the k and water content of PM_(2.5) in Beijing were estimated utilizing the method proposed in this study. The annual average value of k of PM_(2.5) in Beijing was 0.25±0.09, the maximum k value 0.26±0.08 appeared in summer, and the seasonal variation is insignificant. The PM_(2.5) water content was determined by both the PM_(2.5) hygroscopicity and the ambient relative humidity(RH). The annual average mass ratio of water content and PM_(2.5) was 0.18±0.20, and the maximum value 0.31±0.25 appeared in summer. Based on the estimated water content of PM_(2.5) in Beijing, the relationship between the PM_(2.5) water content and RH was parameterized as: m(%)=0.03+(5.73×10~(-8)) ×RH~(3.72).This parametric formula helps to characterize the relationship between the PM_(2.5) mass concentration and atmospheric visibility.  相似文献   

7.
This paper establishes the kinetic equations in atmospheric chemistry that describe the macroscopic mechanisms of secondary fine particle pollution generated by precursors during atmospheric self-purification.The dynamic and static solutions of these equations can be applied to calculate quantitative relationships between the concentration ratio of precursors and secondary fine particles as well as the physical clearance power of the atmosphere,chemical reaction rate,and the scale of a contaminated area.The dynamic solution presented here therefore corresponds with a theoretical formula for calculating the overall rate constant for the oxidation reaction of reducing pollutants in the actual atmosphere based on their local concentrations and meteorological monitoring data.In addition,the static solution presented in this paper reveals the functional relationship between the concentration of secondary fine particles and precursor emission rate as well as atmospheric self-purification capacity.This result can be applied to determine the atmospheric environmental capacity of a precursor.Hourly records collected over the last 40 years from 378 weather stations in mainland China as well as the spatiotemporal distribution sequence of overall oxidation reaction rates from precursors show that when the reference concentration limit of secondary fine particles is100μmol m~(-3),the atmospheric environmental capacity of total precursors canbe calculated as 24890×10~(10) mol yr~(-1).Thus,when the annual average concentration limit of given fine particles is 35μg m~(-3) and the ratio of sulfate and nitrate to 30% and 20% of the total amount of fine particles,the capacities of SO_2,NO_x and NH_3 are 1255,1344,and 832(10~(10)g yr~(-1)),respectively.The clearance density of precursors for different return periods across mainland China under above conditions are also provided in this study.  相似文献   

8.
Study of ozone “weekend effect” in Shanghai   总被引：6，自引：0，他引：6  
Analysis of observed ozone data in 2006 from five monitoring sites (Xujiahui, Chongming, Baoshan, Pudong, Jinshan) in Shanghai reveals that ozone (O_3) concentrations in Xujiahui are higher at week-ends than those on weekdays, despite the fact that emissions of ozone precursor substances, such as oxides of nitrogen (NOx), carbon monoxide (CO) and volatile organic compounds (VOCs) are lower at weekends than those on weekdays. The possible chemical cause of ozone "weekend effect" is that NO_2/NO ratio increases at weekends by 25.61% compared with those on weekdays. In addition, because of an average 12.13% reduction in NOx (NO NO_2) in the early morning (05:00-09:00) at weekends compared with that on weekdays, the ozone inhibition period ends 0.5 h earlier at weekends resulting in the longer duration of ozone accumulation and the higher ozone production rate. The rate of ozone production is a function of VOCs and NOx in the atmosphere. VOCs/NOx ratio in Xujiahui is 4.55 at weekends, and 4.37 on weekdays, belonging to the "NOx-limited". The increasing VOCs/NOx ratio at weekends leads to ozone enhancement from 73 ppbv to 80 ppbv, which are consistent with ozone "weekend effect" in Xujiahui. Furthermore, combining with MICAPS cloud amount data, the fact that ozone "weekend effect" in Xujiahui weakens gradually along with the increasing of cloud amount indicates that ozone photochemical production leads to ozone "weekend effect" in Xujiahui of Shanghai.  相似文献   

9.
High-biomass red tides occur frequently in some semi-enclosed bays of Hong Kong where ambient nutrients are not high enough to support such a high phytoplankton biomass. These high-biomass red tides release massive inorganic nutrients into local waters during their collapse. We hypothesized that the massive inorganic nutrients released from the collapse of red tides would fuel growth of other phytoplankton species. This could influence phytoplankton species composition. We tested the hypothesis using a red tide event caused by Mesodinium rubrum(M. rubrum) in a semi-enclosed bay, Port Shelter. The red tide patch had a cell density as high as 5.0×10~5 cells L~(-1), and high chlorophyll a(63.71 μg L~(-1)). Ambient inorganic nutrients(nitrate:NO_3~-, ammonium: NH_4~+, phosphate: PO_4~(3-), silicate: SiO_4~(3-)) were low both in the red tide patch and the non-red-tide patch(clear waters outside the red tide patch). Nutrient addition experiments were conducted by adding all the inorganic nutrients to water samples from the two patches followed by incubation for 9 days. The results showed that the addition of inorganic nutrients did not sustain high M. rubrum cell density, which collapsed after day 1, and did not drive M. rubrum in the non-red-tide patch sample to the same high-cell density in the red tide patch sample. This confirmed that nutrients were not the driving factor for the formation of this red tide event, or for its collapse. The death of M. rubrum after day 1 released high concentrations of NO_3~-,PO_4~(3-), SiO_4~(3-), NH_4~+, and urea. Bacterial abundance and heterotrophic activity increased, reaching the highest on day 3 or 4, and decreased as cell density of M. rubrum declined. The released nutrients stimulated growth of diatoms, such as Chaetoceros affinis var. circinalis, Thalassiothrix frauenfeldii, and Nitzschia sp., particularly with additions of SiO_4~(3-) treatments, and other species. These results demonstrated that initiation of M. rubrum red tides in the bay was not directly driven by nutrients.However, the massive inorganic nutrients released from the collapse of the red tide could induce a second bloom in low-ambient nutrient water, influencing phytoplankton species composition.  相似文献   

10.
Freezing can increase the emissions of carbon dioxide(CO_2) and nitrous oxide(N_2O) and the release of labile carbon(C) and nitrogen(N) pools into the soil. However, there is limited knowledge about how both emissions respond differently to soil freezing and their relationships to soil properties. We evaluated the effect of intensity and duration of freezing on the emissions of CO_2 and N_2 O, net N mineralization, microbial biomass, and extractable C and N pools in soils from a mature broadleaf and Korean pine mixed forest and an adjacent secondary white birch forest in northeastern China. These soils had different contents of microbial biomass and bulk density. Intact soil cores of 0–5 cm and 5–10 cm depth sampled from the two temperate forest floors were subjected to -8, -18, and -80°C freezing treatments for a short(10 d) and long(145 d) duration, and then respectively incubated at 10°C for 21 d. Soil cores, incubated at 10°C for 21 d without a pretreatment of freezing, served as control. Emissions of N_2 O and CO_2 after thaw varied with forest type, soil depth, and freezing treatment. The difference could be induced by the soil water-filled pore space(WFPS) during incubation and availability of substrates for N_2 O and CO_2 production, which are released by freezing. A maximum N_2 O emission following thawing of frozen soils was observed at approximately 80% WFPS, whereas CO_2 emission from soils after thaw significantly increased with increasing WFPS. The soil dissolved organic C just after freezing treatment and CO_2 emission increased with increase of freezing duration, which paralleled with a decrease in soil microbial biomass C. The cumulative net N mineralization and net ammonification after freezing treatment as well as N_2 O emission were significantly affected by freezing temperature. The N_2 O emission was negatively correlated to soil p H and bulk density, but positively correlated to soil K_2SO_4-extractable NO_3~--N content and net ammonification. The CO_2 emission was positively correlated to the cumulative net N mineralization and net ammonification. From the above results, it can be reasonably concluded that for a wide range of freezing temperature and freezing duration, N_2 O and CO_2 emissions after thaw were associated mainly with the changes in soil net N mineralization and the availability of substrate liberated by freezing as well as other soil properties that influence porosity.  相似文献   

11.
The investigation and continuous monitoring with an innovative iron oxide embedded cellulose acetate membrane (FeO/CAM) on the concentrations of biologically available phosphorus (BAP) were conducted in the Meiliang Bay of the Taihu Lake during summer in 2004. The results showed that the concentrations of dissolved (FeO-DP), particulate (FeO-PP) and total bioavailable phosphorus (FeO-P) had similar horizontal distribution. The BAP concentrations were the highest in those estuaries in the northern bay. With the decrease of the distance to the estuary or long shore, there was little difference between BAP concentrations in an open lake area. During the observation period, algal blooms occurred in most waters of the northern bay, which was reflected from the high concentrations of chlorophyll a (Chl-a). While they were not highest in the estuarine waters of those major rivers, this is the case for the BAP concentrations. The concentrations of Chl-a had a significantly positive correlation with those of bioavailable phosphorus in the open area of the Meiliang Bay. With the sediment resuspension induced by wind and wave, BAP concentrations increased in a short-term, indicating that the riverine P inputs mainly contribute to the concentrations of BAP in the estuarine water while internal P release was the major source of BAP in the open lake area. In the eutrophic shallow lake, the blooms of alga may cause pH increase and further result in internal P release. The above results showed that the new membrane of FeO/CAM can be used to monitor the concentrations of BAP and provide the scientific justifications for the control strategy of the lake eu-trophication.  相似文献   

12.
To assess the effects of river damming on dissolved inorganic carbon in the Jialing River, a total of 40 water samples, including inflow, outflow, and stratified water in four cascade reservoirs(Tingzikou, Xinzheng,Dongxiguan, Caojie) were collected in January and July,2016. The major cations, anions, and δ~(13)C_(DIC) values were analyzed. It was found that the dissolved compositions are dominated by carbonate weathering, while sulfuric acids may play a relatively important role during carbonate weathering and increasing DIC concentration. Different reservoirs had variable characteristics of water physiochemical stratification. The DIC concentrations of reservoir water were lower in summer than those in winter due to the dilute effects and intensive aquatic photosynthesis, as well as imported tributaries. The δ~(13)C_(DIC) values in Tingzikou Reservoir were higher during summer than those in winter,which indicated that intensive photosynthesis increased the δ~(13)C_(DIC) values in residual water, but a similar trend was not obvious in other reservoirs. Except for in Xinzheng Reservoir, the δ~(13)C_(DIC) values in inflow and outflow reservoir water were lower than those in the surface water of stratified sampling in summer. For stratified sampling, it could be found that, in summer, the Tingzikou Reservoir δ~(13)C_(DIC) values significantly decreased with water depthdue to the anaerobic breakdown of organic matter. The significant correlation(p0.01 or 0.05) between the DIC concentrations, the δ~(13)C_(DIC) values and anthropogenic species(Na~++K~+, Cl~–, SO_4~(2-) and NO_3~-) showed that the isotope composition of DIC can be a useful tracer of contaminants. In total, Tingzikou Reservoir showed lacustrine features, Xinzheng Reservoir and Dongxiguan Reservoir had "transitional' features, and Caojie Reservoir had a total of "fluvial' features. Generally, cascade reservoirs in the Jialing River exhibited natural river features rather than typical lake features due to characteristics of reservoir water in physiochemical stratification, spatiotemporal variations of DIC concentrations and isotopic compositions. It is evident that the dissolved inorganic carbon dynamics of natural rivers had been partly remolded by dam building.  相似文献   

13.
The Jialingjiang River basin is one of the main sediment contributing areas in the upper reaches of the Changjiang River. Great changes have taken place in the runoff and sediment discharge in recent years. Comparing the data of 1991-2003 with the data of 1954-1990, the annual runoff of the Jialingjiang River basin decreased by 23 %, and the suspended sediment transport decreased by 74% or 105 million tons. The main factors affecting the reduction include a decrease in rainfall, sediment detention of hydraulic structures, soil and water conservation activities, sedimentation and sand dredging in the river channel. Thorough investigation and analysis of the contribution of each factor to the sediment decrease at Beibei Station was determined for the first time. The following are the contributing percentages for each factor: a decrease in runoff accounted for 32.9%; soil and water conservation measures accounted for 16.4%; sediment detention of hydraulic structures accounted for 30.5%; sedimentation, river channel sand dredging, and other factors accounted for 20.2%. These findings are very important for forecasting the trend of inflow sediment discharge variation.  相似文献   

14.
Based on the Weather Research and Forecasting model and the Models-3 community multi-scale air quality model(WRF-CMAQ),this study analyzes the impacts of meteorological conditions and changes in air pollutant emissions on the heavy air pollution episode occurred over North China around the 2020 Spring Festival(January to Februray 2020).Regional reductions in air pollutant emissions required to eliminate the PM2.5 heavy pollution episode are also quantified.Our results found that meteorological conditions for the Beijing-Tianjin-Hebei and surrounding"2+26"cities are the worst during the heavy pollution episode around the 2020 Spring Festival as compared with two other typical heavy pollution episodes that occurred after 2015.However,because of the substantial reductions in air pollutant emissions in the"2+26"cities in recent years,and the32%extra reduction in emissions during January to February 2020 compared with the baseline emission levels of the autumn and winter of 2019 to 2020,the maximum PM2.5 level during this heavy pollution episode around the 2020 Spring Festival was much lower than that in the other two typical episodes.Yet,these emission reductions are still not enough to eliminate regional heavy pollution episodes.Compared with the actual emission levels during January to February 2020,a 20%extra reduction in air pollutant emissions in the"2+26"cities(or a 45%extra reduction compared with baseline emission levels of the autumn and winter of 2019 to 2020)could help to generally eliminate regionwide severe pollution episodes,and avoid heavy pollution episodes that last three or more consecutive days in Beijing;a 40%extra reduction in emissions(or a 60%extra reduction compared with baseline emission levels of the autumn and winter of 2019 to 2020)could help to generally eliminate regionwide and continuous heavy pollution episodes.Our analysis finds that during the clean period after the heavy pollution episode around the 2020 Spring Festival,the regionwide heavy pollution episode would only occur with at least a 10-fold increase in air pollutant emissions.  相似文献   

15.
Recent works reveal that the size reduction of or- ganisms during the Permian-Triassic transition is of great importance for research on biotic mass extinction and recovery in this period[1,2]. Initially, Urbanek (1993) observed a decrease in the size of Silurian graptolites during the biotic crisis, and used the term “Lilliput Effect” to define the size reduction in sur- viving animal taxa[3]. Subsequently, researchers re- ported a decrease in size of late Devonian conodonts[4], heart urc…  相似文献   

16.
How to mitigate anthropogenic carbon emissions in cities determines to a large degree whether global temperature targets in this century are to be met. Using 12 cities in or outside China as case studies, we quantified the critical processes of carbon metabolism based on the urban carbon metabolism assessment framework(CMAF) proposed. The differences of sector contribution, and per capita and intensity among carbon throughflows, carbon inflows and carbon emissions were evaluated.Furthermore, we established an indicator system for CMAF consisting of flow-based and structural indicators to compare the low-carbon performances of cities. The results showed that the total carbon throughflow(TCT) and total carbon inflow(TCI) in Chinese cities were 7–12% higher than in European and American cities regarding the manufacturing and services sector on average, but 6–9% lower in the household consumption sector. Beijing, Tianjin, Nanjing and Guangzhou had lower per capita TCT and TCI than in European and American cities such as Paris and Los Angeles, while their carbon intensities were about three times as much. The per capita TCT in a city was found significantly correlated with per capita energy consumption and had a certain correlation with per capita building or housing area. This study found that TCT, TCI and carbon dioxide emission each provided unique information to measure the potential climatic impact of cities. The difference in the ranking of low-carbon performance between the investigated cities was significant both in terms of flow-based and structural indicators. We suggest these assessment indicators of carbon metabolism be integrated into urban resources management to reflect both the decarbonization status and future emission reduction potential more accurately and to provide systemic decision support for achieving the goal of carbon neutrality in cities.  相似文献   

17.
Atmospheric SO_2 has a significant impact on the urban environment and global climate. Band Residual Difference Algorithm(BRD) and Differential Optical Absorption Spectroscopy(DOAS) were used respectively by NASA and ESA science team to derive SO_2 columns from satellite observations, but there are few studies on the comparison and validation of BRD and DOAS SO_2 retrievals under the same observation conditions. In this study, the radiative transfer model SCIATRAN was firstly used to validate the accuracies of BRD and DOAS SO_2 retrievals, and analyse the uncertainty of SO_2 retrieval caused by band selection,O_3 absorption, aerosol, surface reflectance, solar and viewing zenith angle. Finally, BRD and DOAS algorithms were applied to the same radiances from satellite observations, and comparisons of BRD and DOAS SO_2 retrievals were conducted over volcanic eruption and North China. Results show that, for the case with low SO_2 columns, BRD SO_2 retrievals have higher retrieval accuracy than DOAS, but typical seasonal variation with high SO_2 column in winter and low in summer can be more clearly discernible in DOAS SO_2 retrievals than BRD from satellite observations. For the case with high SO_2 columns, the differences between BRD(310.8–314.4 nm) and DOAS(315–327 nm) retrievals are large, and the value and accuracy of BRD(310.8–314.4 nm) SO_2 retrievals are lower than those of DOAS(315–327 nm) retrievals. Compared with the SO_2 inputs in forward model, both BRD(310.8–314.4 nm) and DOAS(315–327 nm) SO_2 retrievals are underestimated for the case with high SO_2 columns. The selection of wavelength range can significantly affect the accuracy of SO_2 retrieval. The error of BRD SO_2 retrieval from 310.8–314.4 nm is lower than other bands in the ultraviolet spectral region(306–327 nm). The increase of wavelength in the ultraviolet spectral region306–330 nm can reduce the underestimation of DOAS SO_2 retrievals in the case of high SO_2 column, but slight overestimation of SO_2 retrieval is found from the 315–327 nm range in the case of low SO_2 column. The values of BRD and DOAS SO_2 retrieval decrease with atmospheric O_3 column and aerosol optical depth increasing, but increase with surface reflectance increasing. Large solar zenith angle and viewing zenith angle can introduce more errors to the BRD and DOAS SO_2 retrievals. This study is important for the improvement of retrieval algorithm and the application of SO_2 products from satellite observations.  相似文献   

18.
As an earthquake-prone country, China has made sustained efforts in the study of earthquakes and disaster mitigation during the past several decades, with China Seismological Bureau (CSB) as the backbone of these efforts. Working towards this purpose, a series of key projects were implemented in the “Ninth Five-Year Plan” (1995-2000) to upgrade earthquake monitoring systems and to improve the supporting infrastructure, significant results in earthquake science were achieved. In the new century, we have worked out a blueprint for earthquake preparedness and disaster mitigation in the “Tenth Five-Year Plan”, which emphases 3 systems (i.e. Seismic Monitoring & Prediction, Seismic Hazards Prevention, Emergency Response), and 10 key projects in earthquake science and technology.  相似文献   

19.
The significance of the various biogeochemical pathways that drive carbon cycling and the relative fractions of dissolved inorganic carbon(DIC) produced by these reactions within the sulfate-methane transition zone(SMTZ) are still being debated. Unraveling these processes is important to our understanding of the benthic DIC sources and their contributions to the global carbon cycle. Here, we measure pore water geochemistry(chlorine, sulfate, methane, Ca~(2+), Mg~(2+), DIC and δ~(13)C-DIC) as well as solid geochemistry(sedimentary organic carbon(SOC) and δ~(13)C of SOC) in nearshore sediments from Qi'ao Island in the Pearl River Estuary of the Southern China Sea. Our analysis indicates that SOC originates from the mixing of carbon from terrestrial and marine sources, and that terrestrial materials dominate the net loss of SOC during the degradation of organic matter, especially at sites located near the river outlets. Sulfate reduction via SOC degradation is not appreciable in the upper sediment layer due to conservative mixing-dilution by freshwater. However, below this layer, the anaerobic oxidation of methane(AOM) and methanogenesis occur. Within the SMTZ, the δ~(13)C mass balance shows that the proportions of DIC derived from organoclastic SO_4~(2-) reduction(OSR) and AOM are 50.3% to 66.7% and 0.1% to 17.9%, respectively, whereas methanogenesis contributes 17.0% to 43.9%. This study reveals that the upward diffusion of DIC from ongoing methanogenesis significantly influences carbon cycling within the SMTZ in these estuarine sediments. As a result, we suggest that the plots of the ratio of change in sulfate to change in DIC in pore water should be used with caution when discriminating between sulfate reduction pathways in methane-rich sediments.  相似文献   

20.
Changes in monsoon precipitation have profound social and economic impacts as more than two-thirds of the world's population lives in monsoon regions. Observations show a significant reduction in global land monsoon precipitation during the second half of the 20 th century. Understanding the cause of this change, especially possible anthropogenic origins, is important.Here, we compare observed changes in global land monsoon precipitation during 1948–2005 with those simulated by 5 global climate models participating in the Coupled Model Inter-comparison Project-phase 5(CMIP5) under different external forcings.We show that the observed drying trend is consistent with the model simulated response to anthropogenic forcing and to anthropogenic aerosol forcing in particular. We apply the optimal fingerprinting method to quantify anthropogenic influences on precipitation and find that anthropogenic aerosols may have contributed to 102%(62–144% for the 5–95% confidence interval)of the observed decrease in global land monsoon precipitation. A moisture budget analysis indicates that the reduction in precipitation results from reduced vertical moisture advection in response to aerosol forcing. Since much of the monsoon regions,such as India and China, have been experiencing rapid developments with increasing aerosol emissions in the past decedes, our results imply a further reduction in monsoon precipitation in these regions in the future if effective mitigations to reduce aerosol emissions are not deployed. The observed decline of aerosol emission in China since 2006 helps to alleviate the reducing trend of monsoon precipiptaion.  相似文献   

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